Charge carriers with fractional exclusion statistics in cuprates
P. A. Marchetti, F. Ye, Z. B. Su, L. Yu

TL;DR
This paper demonstrates that charge carriers in cuprates can be described with fractional exclusion statistics, explaining experimental features and Fermi volume behavior in high-temperature superconductors.
Contribution
It introduces a consistent application of fractional exclusion statistics to charge carriers in cuprates within a gauge approach, linking theory to experimental observations.
Findings
Charge carriers exhibit exclusion statistics with parameter 1/2.
Large Fermi volume of holes at high doping levels.
Natural explanation for unusual properties of hole-doped cuprates.
Abstract
We show that in the SU(2)XU(1) spin-charge gauge approach we developed earlier one can attribute consistently an exclusion statistics with parameter 1/2 to the spinless charge carriers of the t-J model in two dimensions(2D), as it occurs in one dimension (1D). Like the 1D case, the no-double occupation constraint is at the origin of this fractional exclusion statistics. With this statistics we recover a "large" Fermi volume of holes at high dopings, close to that of the tight binding approximation. Furthermore, the composite nature of the hole, made of charge and spin carriers only weakly bounded, can provide a natural explanation of many unusual experimental features of the hole-doped cuprates.
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Charge carriers with fractional exclusion statistics in cuprates
P. A. Marchetti
Dipartimento di Fisica e Astronomia, INFN, I-35131 Padova, Italy
F. Ye
Department of Physics, Southern University of Science and Technology, Shenzhen 518055, China
Z. B. Su
Institute of Theoretical Physics, Chinese Academy of Sciences, 100190 Beijing, China
L. Yu
Institute of Physics, Chinese Academy of Sciences,and Beijing National Laboratory for Condensed Matter Physics, 100190 Beijing, China
University of Chinese Academy of Sciences, 100049 Beijing, China
Abstract
We show that in the spin-charge gauge approach we developed earlier one can attribute consistently an exclusion statistics with parameter 1/2 to the spinless charge carriers of the - model in two dimensions (2D), as it occurs in one dimension (1D). Like the 1D case, the no-double occupation constraint is at the origin of this fractional exclusion statistics. With this statistics we recover a ”large” Fermi volume of holes at high dopings, close to that of the tight binding approximation. Furthermore, the composite nature of the hole, made of charge and spin carriers only weakly bounded, can provide a natural explanation of many unusual experimental features of the hole-doped cuprates.
pacs:
71.10.Hf, 11.15.-q, 71.27.+a
I Introduction
Despite continuous experimental advances it has not yet been obtained an agreement on the interpretation of the low-energy physics of cuprates; see, , Ref. uchida, for an excellent, state-of-the-art review. A general consensus has been achieved, however, that most of the relevant phenomena in hole-doped materials can be derived from modeling the CuO planes in these materials in terms of a two-dimensional (2D) - model on the copper sites with the Hamiltonian:
[TABLE]
where denotes the nearest neighbour (NN) sites, the hole field operator with spin index on site , the Gutzwiller projection eliminating double occupation, and summation over repeated spin (and vector) indices is understood hereafter. The Gutzwiller projected holes describe the Zhang-Rice singlets zr of cuprates.
A way of implementing the Gutzwiller projection is to apply to fermions of the model a spin-charge decomposition formalism. It has been pioneered by Anderson an and Kivelson kiv and it is suggested for cuprates by the rather different response of charge and spin degrees of freedom in many experiments: One rewrites the fermion field as a product of a spinless holon field carrying the charge degree of freedom and a spin 1/2 spinon field carrying the spin degree of freedom, imposing on them a constraint reproducing the Gutzwiller projection. Due to this decomposition an emergent (slave-particle) gauge symmetry appears, since holon and spinon fields can be multiplied by factors with opposite phases leaving the original fermion field unchanged. For this reason only slave-particle gauge-invariant fields are physical and therefore neither the holon nor the spinon by themselves are physical and they are strongly coupled by gauge fluctuations. However, by gauge-fixing this gauge symmetry one can consider gauge-dependent fields, which may be convenient in the description of at least some momentum-energy range, as gluons and quarks in high-energy QCD, in spite of the fact that only mesons and baryons are physical in strict sense. It makes sense then to discuss the statistics of holon and spinon fields and of the ”quasi-particle” excitations, in this generalized sense, that they might generate in the low-energy limit. This is a key issue of this article. Notice that the spin-charge decomposition formalism does not prohibit a priori that the fermion field describes an elementary excitation without a composite structure, as it happens e.g. for the meson field written in terms of quark fields in lattice QCD in the ”super-confining phase”, as discussed in Ref. frobri, . Whether the fermion excitation described by is composite or not is a dynamical question, it does not have a purely kinematical character as, on the contrary, the spin-charge decomposition does. Somewhat related considerations on the kinematical character of the spin-charge decompositions versus the dynamical character of their low-energy excitations can be found in Ref. lee, .
As rigorously shown in Ref. fro, , spin-charge decomposition can be achieved in the Lagrangian formalism by coupling the original fermions with suitably chosen Chern-Simons gauge fields. Furthermore, one may change the braid statistics of holons and spinons, while still keeping the Fermi statistics of the original holes. Different choices of Chern-Simons actions precisely reflect these different braid statistics.
In one- and two-dimensions abelian braid statistics of particles (or of field operators that create them) can be characterized by the phase factor acquired by their many-body wave-function (or the product of equal-time field operators) when one performs an oriented exchange among two of them, with and referring to the two orientations (see, , Ref. wil, ). Fermions(bosons) correspond to (1), while excitations with are called semions.
All appropriate choices of holon and spinon statistics reproduce exactly the correlation functions of the original fermion fields, as shown in the specific examples of slave bosons, slave fermions and slave semions in Refs. fro, , and using techniques developed there many more schemes can be employed, , the slave anyons considered in Ref. ls, or a variant of the slave semion approach considered in Ref. msy98, , on which our subsequent discussion is based. Slightly different roads follow, , the approach of Ref. wlmw, , as commented in this spirit in Ref. msy, .
Although all Chern-Simons choices are completely equivalent if implemented exactly, as soon as one makes some mean-field-like approximation they give rather different resultsmsy . It is then crucial to understand which choice is better to perform mean-field treatments. As discussed below, a key issue is the area (2D volume) of the Fermi surface and that issue is in turn closely linked to another form of statistics for the elementary excitations of the model, , the .
The exclusion statistics was introduced by Haldane ha to generalize the Pauli exclusion principle. It can be characterized at finite density by the average occupation of momenta at as follows wu : Consider a Fermi gas with fixed “volume” (in 2D later on called area) enclosed by the Fermi surface and let be the corresponding fermion density; we say that a particle obeys exclusion statistics with parameter if the particle density with the same Fermi “volume”, denoted by , satisfies
[TABLE]
This implies that at a fixed momentum (neglecting other internal degrees of freedom) a particle with exclusion statistics 1/2 can have an occupation number twice that of a free fermion, so that the “volume” of its Fermi surface is half of that of a Fermi gas with the same density. In a “cartoon language” one might say that a semion in momentum space behaves like “one half” of a fermion.
For the statistics of “quasi particle” excitations of the 2D - model and the related Fermi surface area we have two sources of suggestions: The solvable one-dimensional (1D) - model and, under the assumption initially made, the experiments on cuprates.
Concerning the 1D model the answer for the braid statistics is unique: Both holon and spinon fields and the related low-energy ”quasi-particles” should be semions, , with braid statistics parameter , to reproduce in a suitable mean-field treatment the correct scaling limit of correlation functions obtained via Bethe ansatz or conformal field theory methods haha ; np .
Furthermore, the holon in 1D has exclusion statistics parameter . As shown in Ref.ymsy, , in general there is no relation between the braid and exclusion statistics in 1D. In fact one can introduce the braid statistics coupling 1D spinless fermions to a Chern-Simons field and then perform its dimensional reduction. The physical gauge-invariant field is obtained by adding to the fermion field a gauge string and it obeys a braid statistics consistent with the Chern-Simons coefficient. The Fermi points are shifted by the gauge string but the Fermi 1D “volume” remains constant, hence the corresponding low-energy excitations still obey an exclusion Fermi statistics. A non-trivial exclusion statistics emerges if the fermionic fields have a Luttinger interaction, a connection previously clearly stated in Ref. wy, . In the approach of Ref. np, to the 1D - model, neglecting at first the coupling with spinons, the holon at large scale behaves as a free U(1) semion; spinons are described by Gutzwiller projected fermions in a squeezed chain obtained by omitting the holon sites and at large scale they form a semion gas with exclusion parameter described effectively by a Luttinger liquid theory. We then perform a field redefinition, eliminating the Fermi surface for the spinon fields by suitably stripping away their gauge strings and adding them to the holon in the correlation functions of the physical hole. As result the 1/2 exclusion statistics of spinons is transferred to holons; holons then have , so that the Fermi momentum of the U(1) semionic holon equals the Fermi momentum of the original spin 1/2 fermion treated in the tight binding approximation, in agreement with the exact solution of the model. In fact in such exact solution the Fermi points of the hole are in the position expected for a spin 1/2 fermion with the standard Pauli principle, consistently with the Luttinger theorem, as extended to 1D Luttinger liquids in Ref. yoa, . Since in the spin-charge decomposition spinons with the above redefinition don’t have a Fermi surface while holons are spinless, that result is correctly recovered by the 1/2 exclusion statistics of holons.
We now turn to the suggestion coming from experiments on cuprates. In overdoped materials the Fermi surface seen in ARPES is close to that obtained in a tight-binding approximation of a -- model and satisfies the standard Luttinger theorem. (The introduction of a next nearest neighbor (NNN) hopping parameter , and possibly a NNNN , in the formalism discussed here is straightforward and it does not change the qualitative features, so it will not be elaborated anymore). To reproduce this result in the spin-charge decomposition formalism we have two natural options: Either the spin 1/2 spinon is fermionic with Fermi surface and the holon is a hard-core boson, as in the slave-boson approach (see, . Ref. lee, ), or the spinless holon has Fermi surface with exclusion statistics parameter 1/2, hence with the same Fermi surface of spinons of the slave-boson approach, while the spinon has no Fermi surface.
We see that, if both spinon and holon are semions, the second case would be a close analogue to what happens in 1D. We remarked above that in 1D the natural condition for the appearance of exclusion statistics is the Luttinger interaction; analogously on general grounds we proved in Ref. ym, that in 2D we have if the original fermionic system without Chern-Simons coupling has Hall conductivity 1/2 and is incompressible. The main goal of this paper is to show that indeed these conditions can be satisfied for the holon in the 2D model and the second approach considered above to get the correct Fermi area can be consistently implemented, sketching also a derivation from it of some consequences for cuprates.
II The spin-charge gauge approach
To implement a semionic decomposition of the hole in the 2D - model we start by making use of the following theorem fro ; np .
Theorem: We embed the lattice of the 2D - model in a 3-dimensional space, denoting by coordinates of the corresponding 2+1 space-time, being the euclidean time. We couple fermions of the - model to a gauge field, , gauging the global charge symmetry, and to an gauge field, , gauging the global spin symmetry of the model, and we assume that the dynamics of the gauge fields is described by the Chern-Simons actions with:
[TABLE]
where is the Levi-Civita anti-symmetric tensor in three dimensions. Then the spin-charge (or ) gauged model so obtained is exactly equivalent to the original - model. In particular the spin and charge invariant correlation functions of the fermion fields of the - model are exactly equal to the correlation functions of the fields , where denotes now the fermion field of the gauged model, a string at constant euclidean time connecting the point to infinity and the path-ordering, which amounts to the usual time ordering , when “time” is used to parametrize the curve along which one integrates. One can view the result of this theorem as an analogue of the construction of composite fermions in Jain’s approach to the Quantum Hall Effect jain . In that case magnetic vortices with even quantum flux (depending on the filling) are bound to the electron and the resulting composite entity is still a fermion, dubbed composite fermion; in the present case the electron of the - model is bound to a charge-vortex of flux -1/2 and a spin-vortex of flux 1/2, while the resulting entity still being a fermion.
Notice that, contrary to what one might naively think, although the Chern-Simons actions individually explicitly break the parity and time-reversal symmetries, the particular combination considered above still preserves explicitly these two symmetries.
We now rewrite the hole field of the gauged model as a product of a charge 1 spinless fermion field and a neutral spin 1/2 boson field : . Then we identify as the holon and as the spinon fields. The Chern-Simons coupling automatically ensures that both corresponding field operators obey semionic braid statistics. The holon being spinless implements exactly the Gutzwiller constraint due to the Pauli principle. Furthermore, if the constraint is imposed, as we see that is just the density of empty sites in the model, corresponding to the Zhang-Rice singlets.
The ”charge-flux” associated to the electrons produces a -flux phase for every plaquette, plus vortices centered on the empty sites, on the holon positions. More precisely, introducing a Coulomb gauge-fixing for the charge gauge symmetry, one finds
, where
[TABLE]
and we can choose
[TABLE]
where is a site of the even Néel sublattice and the two unit vectors along the link directions. We recognize as the vector potential of a vortex centered at the holon position , , centered at an empty site of the - model. Vortices in Eq. (II.2) appear in the charge group and are responsible for the semionic nature of holons.
Neglecting at first these charge-vortices, through Hofstadter mechanism the -flux converts the spinless holon field into a pair of “Dirac fields” in the magnetic Brillouin zone (BZ), with pseudospin indices corresponding to the two Néel sublattices and two “small FS” centred at . If we reinsert the charge-vortices, and assume for the corresponding semionic holons an exclusion statistics 1/2, then these holons have the same FS of the fermionic spinons of the slave-boson approach in the -flux phase lee , and the same dispersion: , where denotes the density of empty sites, corresponding in cuprates to the in-plane doping concentration. When these holons are coupled to spinons through the self-generated slave-particle gauge field, as a consequence of the Dirac structure of the holons the resulting holon-spinon bound state generated in the low-energy limit exhibits Fermi arcs qualitatively consistent with those found in ARPES experiments in the pseudogap “phase” in cuprates msy04 . The underlying FS for the hole is modified the holon FS by the spinon gap proportional to discussed later. Furthermore, using the techniques of Refs.msy04, , mg, and assuming a doping independent renormalization of the spinon gap, the fraction of BZ enclosed can be for all dopings approximately , where the factor 1/2 comes precisely from the 1/2 exclusion statistics mysy .
We can now use the gauge freedom to rotate the spinons to a configuration , depending on the holon configuration, optimizing “on average” the holon-partition function in that spinon background, in a Born-Oppenheimer approximation. In this configuration spinons are antiferromagnetically ordered along the magnetization direction of the undoped model, which we arbitrarily fix along . There is in addition a spin flip on the sites where holons are present, also for the final site of a hopping link of holons, at the time of hopping. Above a crossover temperature we find that involves also a phase factor cancelling the contribution of in the loops of hopping links of holons, so that the hopping holons feel an approximately zero flux msy05 . Assuming the exclusion statistics with parameter 1/2 for the holon (to be proved in the next Section), the disappearance of the -flux implies that the Hofstadter mechanism does not hold anymore and above one recovers for holons the “large FS” of the tight-binding approximation. In particular the fraction of BZ enclosed is of order and the factor 1/2 comes precisely again from the 1/2 exclusion statistics. This FS will be inherited by the physical hole as a holon-spinon bound statemsy05 , and, with the addition of a term and a renormalization of the spinon gap, it is in approximate agreement with the FS observed in ARPES in the ”strange-metal” region of the phase diagram of the cuprates mysy . For this reason we call pseudogap (PG) for the - model in our approach the region below and strange metal (SM) the region above it. Actually, although only qualitatively, the above results on the FS have been proved in Refs. msy04, , msy05, in a rough approximation in which the 1/2 Haldane statistics for the holon was assumed, but, somewhat inconsistently, the semionic nature of the holon field was not taken into account, keeping, on the other hand, the treatment of the spinon consistent with this approximation. As discussed in the introduction the proof of the Haldane statistics of the holon is the main aim of this paper, but this proof needs some more details on the spin-charge approach that we now provide. At the end of the paper some results obtained with this approach, including a non-BCS mechanism for superconductivity, are outlined, making also contact with experiments in cuprates.
Having used the gauge freedom to rotate spinons to the ”optimal” configuration , we need to integrate the gauge field over all its configurations. Therefore, we split the integration over into an integration over a field , satisfying the Coulomb gauge-fixing with and its gauge transformations expressed in terms of an -valued scalar field , , . Notice that .
describes fluctuations of spinons around the ”optimal” configuration and can be written as:
[TABLE]
with satisfying the constraint:
[TABLE]
We will call in the following again “spinons”. Up to now no approximation has been made and the model in terms of , and is still equivalent to the original - model. However, due to the optimization procedure on the spinon, we expect that the configurations of are dominated by small fluctuations around identity. As discussed in Ref. msy, , the spin flip due to the gauge freedom in allows a simultaneous optimization in terms of the spinon both of the and the term in the Born-Oppenheimer approximation considered above, because (neglecting ) appears in the form on links in the term and as and the identity holds. This phenomenon occurs also in 1D and might be the origin of the good mean field approximation for the semionic statistics.
We now briefly discuss a “mean field” approximation essentially based on the conjecture that the fluctuations are small. If we neglect fluctuations in the calculation of (up to an irrelevant field-independent term) one gets ( with ):
[TABLE]
We recognize in the term of Eq.(II.6) the vector potential of a vortex centered at the holon position , with vorticity (or chirality) depending on the parity of . We call these vortices antiferromagnetic (AF) spin vortices, since they record in their vorticity the Néel structure of the lattice. Hence they are still a peculiar manifestation of the AF interaction, like the more standard AF spin waves. As one can see, they are the topological excitations of the subgroup of the original spin group unbroken in the AF phase, along the spin direction of the magnetization.
These vortices are of purely quantum origin, since, like in the Aharonov-Bohm effect, they induce a topological effect far away from the position of the holon itself, where their classically visible field strength is supported. Hence in this approach the empty sites of the 2D - model, mimicking the Zhang-Rice singlets and corresponding to the holon positions, are cores of the AF spin vortices, quantum distortions of the AF spin background. These vortices have no analogue in the slave-boson approach and in our approach are responsible for both short-range AF order, which we now outline since it will be used in the proof of Haldane statistics, and a new pairing mechanism leading to superconductivity, sketched in the final section, referring to Ref. mfsy, for details. Semionic holons dressed by AF spin vortices are similar to semionic holons in 1D with attached a spinon-derived ”spin string”; the role of kinks as topological defects in 1D is replaced by vortices in 2D.
We can write the total action of the system as a sum of a ”spinon action” and a ”holon action” . For our purpose of the spinon action it is enough to know msy98 that in the long wavelength continuum limit it is given by a non-linear model (in form) for spinons describing the continuum limit of the undoped Heisenberg model with an additional coupling between spinons and the AF spin vortices :
[TABLE]
A quenched average, , over positions of centers for spin-vortices yields the following estimate msy98 : . Hence the term (II.7) provides a mass-gap to spinons, converting the long-range AF order of the Heisenberg model, corresponding to zero doping, to short-range AF order at finite dopings; therefore, spinons have no FS. The spinon system behaves as a spin liquid since spinon confinement is avoided by the interaction with the gapless holons. However, in spite of the presence at lattice level of a Chern-Simons term which turns spinons into semions, in the mean-field long-wavelength limit considered involving the coupling to the holons via AF spin vortices, it is not a chiral spin liquid and spinons in the low-energy limit can be considered as spin 1/2 hard-core boson quasi-particles excitations. Although not confined, in the entire system spinons are weakly bound to holons and anti-spinons by slave-particle gauge fluctuations to form the physical composite holes and magnons, respectively.
By making in Eq. (II.7) a mean-field approximation for , instead of what was previously considered for , we obtain the term
[TABLE]
where is the 2D Laplacian. In the static approximation for holons Eq. (II.8) describes a 2D lattice Coulomb gas with charges depending on the Néel sublattices. In particular the interaction is attractive between holons in opposite Néel sublattices, with maximal strength for nearest neighbor sites, along the lattice directions with a -wave symmetry. Putting back coefficients one finds that the coupling constant of this interaction is , which decreases with increasing doping. For 2D Coulomb gases with the above parameters, pairing appears below a temperature . Hence the charge-pairing originates from the attraction between AF spin vortices with opposite chirality, eventually leading to superconductivity as sketched in the final section.
We write now explicitly the holon action, , since its expression is needed in the proof of exclusion statistics. In PG region can be written as:
[TABLE]
The fact that has the same power at both ends of a hopping link is due to the spin-flip generated by . is a gauge field of the -charge group and is a gauge field of the subgroup of the spin group previously selected by choosing the directions of . The factor 2 in the Chern-Simons action is due to a normalization needed passing from to its subgroup. Integrating over and one reproduces the previous description in terms of and . Notice that since coefficients of the Chern-Simons terms for and have opposite sign, at this stage the parity (P) and time-reversal (T) symmetries are still explicitly preserved. Formally this can be seen by rewriting the gauge fields in the combinations and , where is the identity matrix. Holons are coupled only to , so integrating from the Chern-Simons one gets a delta function for the field strength of which is P and T invariant. We argue, however, that the continuum limit should not be taken considering simultaneously the coupling of holons to and , but firstly only to , to make the holon field charge-gauge invariant and to enforce the semionic statistics, and only afterwards introducing the coupling with the spin degrees of freedom.
To summarize in words, in PG describes fermionic lattice holons in the presence of flux per plaquette with attached charge-vortex generated by that turn them into semions, interacting with spinons and the AF spin vortices described by . In SM the flux in the hopping is suppressed.
III The 1/2 exclusion statistics of holons
Having explained the relevance for self-consistency of the exclusion statistics 1/2 for the holon in the spin-charge gauge approach to cuprates, in this Section we turn to its proof.
III.1 The braid-exclusion statistics relation
A key ingredient of the proof is the result contained in Ref. ym, , connecting braid and exclusion statistics under some conditions, that we now sketch.
Consider a planar Hall system consisting of fermions in a thermodynamically large domain with a boundary; it is well known that there are chiral edge modes on the sample boundary leading to a boundary current. We then couple the system to a Chern-Simons field , defined in the whole space-time, with coupling strength , while keeping fixed the chemical potential . We denote by the number of particles contained in the considered domain with Chern-Simons coupling . The Lagrangian (in real time) reads
[TABLE]
where is the current density. The exact form of the Lagrangian of fermions is not so important, and it is only required to provide a non-vanishing Hall conductance .
By differentiating Eq. (III.1) (), one obtains the following relation between the current and the “electric” field: , where is the unit vector perpendicular to the plane of the system. Thus a current flowing on the boundary leads to an electric field normal to the boundary.
In the scaling limit the fermion Hall system contributes a Chern-Simons term to the gauge effective action with coefficient in the bulk (plus a term localized at the boundary by gauge-invariance). Taking into account this contribution in random phase approximation (RPA) leads to an effective Chern-Simons coupling for the field: . The above electric field generated by the boundary current implies a jump of the scalar potential across the sample boundary. Then the change of the free energy due to the Chern-Simons coupling reads
[TABLE]
Differentiating both sides of Eq. (III.2) with respect to , we obtain
[TABLE]
where and is proportional to the compressibility. For an incompressible liquid, one obtains
[TABLE]
Since was kept invariant, by comparing Eq. (III.4) with Eq. (I.2) one concludes that anyons of the system described in Eq. (III.1) obey an exclusion statistics with parameter . In particular, if we have .
Let us now come back to our holon system. The above argument shows that if holons without Chern-Simons coupling to have a Hall conductivity and the system is incompressible, then the semionic holons obtained by coupling with obey exclusion statistics 1/2, as we would like to prove.
III.2 The free holons
In the “holon action” Eq. (II) if no further approximations are made the holon density remains , since the Gutzwiller projection is still exactly implemented by with the constraint Eq. (II.5) being satisfied. In particular when the holon density vanishes, correctly reproducing the vanishing density of Zhang-Rice singlets at half-filling.
However, in the large-scale continuum limit we have seen that, thanks to the interaction with AF vortices, the spinon is gapped. It implies that in this limit the constraint Eq. (II.5) is not fully satisfied, as the spinon mass gap is incompatible with it, so the Gutwiller projection is not anymore exactly implemented. To understand the situation let us first consider the free holons without coupling to spinons and the Chern-Simons fields and , while still keeping fixed the chemical potential. The corresponding action is given by
[TABLE]
Due to the staggered -flux implemented by , we divide the square lattice into two sublattices, A(even sites) and B (odd sites). On these sublattices, the annihilation operators of holons are denoted by and , respectively. Let’s choose a unit cell with A and B sites along the -direction, then the Hamiltonian corresponding to the free holon action Eq. (III.5) can be recast in a quadratic form, with a matrix in the momentum space given by:
[TABLE]
In Eq. (III.6), the momentum only takes values in the range , which is a half of the original BZ. One can easily see that it describes two massless Dirac double-cones with vertices at . Shifting the two Dirac nodes to the origin in -space, inserting the chemical potential and taking the continuum limit, we see that the corresponding continuum fields are described by massless Dirac fields with two flavors, corresponding to the two double-cones. The two upper bands of the double-cones are filled up to energy , hence even at the lower bands of the two Dirac double-cones are filled, so that the holon density no more vanishes even in the half-filling case.
The lower bands are thus an artifact produced by the violation of the constraint Eq. (II.5) introduced when we treat in mean field Eq. (II.7).
Since spinons are gapped, the Gutzwiller constraint is relaxed in the large-scale continuum limit. Going back to the lattice model with no-double-occupation constraint ignored temporarily, one expects that at half filling with the number of holons equals the number of unprojected holes, hence one expects the holon number is 1 per site on average. If these holons were fermions obeying Fermi statistics, both upper and lower bands would be completely filled, which is at odds with the previous half-filling result obtained from the free holon Lagrangian.
This would lead to an inconsistency in the above continuum limit. However, if holons satisfy the semionic exclusion statistics with , at half filling they fill the lower bands leaving the upper bands empty to give a density 1 on average. Since these semionic holons in the lower bands are a result of relaxing the Gutzwiller projection, they are “spurious” and describe the singly occupied sites in the original unprojected lattice model. When the doping holes are introduced in the - model, the corresponding “physical” holons partially fill the upper bands and are responsible for the low energy physics. Although the spurious lower band holons are not directly relevant to the low energy physics in the scaling limit, they are responsible for the 1/2 exclusion statistics when coupled to the statistical field , making the theory self-consistent, as we prove below. Before closing this subsection, we emphasize that one should be careful not introducing an unphysical coupling of the “spurious” holons in the lower bands with spinons, so that the density of “physical” holons coupled to spinons still correctly vanishes at .
III.3 Hall conductivity of ”spurious” holons
According to the strategy outlined in subsection A we now compute the Hall conductivity of the holon system without Chern-Simons couplings. If we look at the corresponding “holon action” in Eq. (II), we see that for sites in the A sublattice and links starting from the A sublattice the coupling with spinons and the field is of the form and , whereas for the B sublattice the corresponding terms are and . Since and , the action is not invariant under time-reversal, but is invariant under time-reversal combined with interchange of the two Néel sublattices realized by parity transformation with respect to a line in the dual lattice. This can be intuitively understood since the time-reversal operation reverses the chirality of the spin-vortices described by , but an exchange of the Néel sublattices also does the same job.
As well known re , to compute the Hall conductivity of massless Dirac fields we need to introduce an infrared regulator (like a mass) with a parameter , respecting the symmetry of the system; at the end of the computation one takes the limit . The reason for introducing a regulator is that, due to the parity anomaly one cannot consistently define a gauge-invariant coupling for massless Dirac fermions in 2D. The mass regulator breaks parity and even after it is sent to zero, in the gauge-effective action its remnant is still there, keeping the information of the mass sign in the coefficient of the generated Chern-Simons action. However, for our system one cannot take as regulator simply a mass term in the lattice as in the standard systems, since it would preserve the time-reversal symmetry, broken in our case.
A regularized free Hamiltonian for the field maintaining the above discussed symmetry has a matrix form in the momentum space given by:
[TABLE]
One can check directly that this Hamiltonian with the regulator added respects the combined symmetry of time reversal and the exchange of Néel lattice of the original Hamiltonian. To be specific the time reversal operation is implemented by complex conjugation and , while the interchange of Néel sublattices corresponds to ( a mirror reflection about the x-axis ) followed by a similarity transformation implemented by . In our units the Hall conductivity of the lower bands is given by , where is the Chern number of the corresponding bands. For a two-dimensional as ours, can be computed as follows (See, , Ref. st, ): We write in terms of , with and the Pauli matrices: . We call the set of points in the BZ where , which are called Dirac points, then
[TABLE]
If we compute the Chern number of the lower bands of , describing “spurious” holons as discussed above, one then finds 1, since at the two Dirac points (becoming for the Dirac nodes) the regulator term has opposite sign : and the second sign in Eq. (III.8) is also opposite at those points. We then see that the lower bands in our holon system contribute to the Hall conductivity.
In order to discuss the spinon coupling to the “physical” upper bands taking into account the gap of spinons, as done in the next subsection, one needs to go to the long-wavelength continuum limit. In that limit the lower bands of the above Hamiltonian are just the lower bands of two Dirac double-cones regularized with the same mass . Since every cone contributes to the Hall conductivity with ,re we see again that the lower bands in our system contribute .
III.4 Hall conductivity of “physical” holons
In the absence of the spinon coupling, for free Dirac holons the partially filled upper bands would contribute exactly the opposite Hall conductivity of the lower bands, since in case of partial filling the Hall conductivity of the free system is zero. Introducing a mass, we get a non-vanishing result only if the chemical potential is in the mass gap, which is not our case. However, the coupling of the upper band to spinons changes the situation.
To discuss the effect of spinon coupling we need to extract an effective action and compute the coefficient of the corresponding Chern-Simons term for the field. This calculation involves a mixing of the upper “physical” and lower “spurious” bands. In order to minimize such mixing, a careful treatment is needed. In fact, we need only consider the mixing in an infinitesimal neighborhood of the Dirac nodes following the procedure outlined below; more details are deferred to the Appendix.
We consider one partially filled Dirac double-cone, while the other one can be treated in the same way. To identify the Green function of the continuum fields associated with the two bands we start with rewriting the relevant free Dirac propagator with chemical potential at in the following form: let with denote the 2+1 Dirac gamma matrices and the 3-momentum.
Then we findsu ,:
[TABLE]
Naively the first term corresponds to the lower band, but to take into account the problem of mixing quoted above we extend the first term up to a small cutoff with to include the bottom of the upper band, replacing by and subtracting the corresponding contribution in the second term of Eq. (III.4). Note that is eventually sent to zero, after the limit has been taken. Hence the introduction of the small cutoff takes into account only the contribution from the conduction band edge. Since the relevant contribution for physical holons at large scales comes only from the region near the Fermi surface, it is unmodified by the above operation. According to the previous discussion we then insert in the modified second term (assumed to describe the “physical” holons) the minimal coupling to , to spinons and to , whereas we insert only the minimal coupling to in the modified first term describing the “spurious” holons appeared with the violation of the Gutzwiller projection.
We have already calculated above the Hall conductivity of the first term, ; correspondingly the leading contribution in the long wavelength continuum limit of the effective action is given by the Chern-Simons term . We now discuss the Hall conductivity of the second term.
The long wavelength continuum limit of the spinon interaction is just the minimal coupling of holons to the slave-particle gauge field . This is the gauge field of the CP1 representation of the O(3) spinon model, implementing in the continuum the slave-particle gauge invariance. Then the leading term of the effective action due to “physical” holons turns out to be , as shown in the appendix.
We now need to integrate to find both Hall conductivity and, as required by Eq. (III.1), the compressibility of the holon system. The compressibility is proportional to the scalar polarization bubble evaluated at zero energy in the limit of zero momenta.
Since the upper band is partially filled, the leading contribution comes from a region near the Fermi surface. Then at in the limit in the Coulomb gauge its polarization bubble matrix is given by:
[TABLE]
where are the density of states at the Fermi energy, the diamagnetic susceptibility and the Hall conductivity, respectively.
As spinons are gapped, integrating them out one obtains a Maxwell effective action for the slave-particle gauge field ; the spinon polarization bubble matrix at is then given by the diagonal matrix
[TABLE]
with the electric and the diamagnetic susceptibility of the spinon system. The scaling analysis presented in Ref. frogoma, based upon a tomographic representation of fermion Green functions suggests that the RPA approximation gives the leading term in the scaling limit of the polarization bubbles of holons in the presence of the Maxwell interaction originated from spinons, described by , since such interaction is of long-range. The polarization bubble of holons dressed by the spinon interaction in RPA in the small limit is then given by
[TABLE]
where the scalar component (corresponding to compressibility) reads
[TABLE]
while the Hall polarization bubble by
[TABLE]
therefore both vanish at , implying that the upper bands of “physical” holons are incompressible and do not contribute to the Hall conductivity for . The origin of incompressibility can be traced back to the unscreened long-range 2D Coulomb repulsion generated by the slave-particle gauge field, due to the spinon gap. Hence it is a consequence of the Gutzwiller constraint, origin of the gauge field, and of the destruction of the Néel order due to the AF vortices introduced by doping.
Since the lower holon bands are completely filled it then turns out that the total holon system before it is coupled to the Chern-Simons -field is incompressible and provides Hall conductivity . Hence, according to the result stated at the beginning of the Section, after coupling with the resulting semionic holons have exclusion statistics parameter 1/2, as we would like to prove.
As seen in the proof, the role of the slave-particle gauge field, as a direct consequence of the no-double occupation constraint, is crucial to obtain the 1/2 exclusion statistics, exactly as in 1D case, where the constraint is also crucial to realize the 1/2 exclusion statistics by producing a Luttinger-type interaction. Notice that incompressibility of the holon liquid does not imply incompressibility of the hole liquid, because the polarization bubble of the hole involves also the renormalization of the gauge propagators due to the holons.
Furthermore, since the Chern-Simons term of does not contain a coupling to one finds that the total Chern-Simons contribution to the effective action of (both “physical” and “spurious”) holons in the bulk is given by . (Also a gauged Wess-Zumino-Novikov-Witten boundary term is generated by gauge invariance wen ,frs .) Therefore, although broken by the system of semionic holons alone, parity and time-reversal symmetries are still explicitly preserved in the holon system couped to the spinon-inherited field. In fact, the bands of “spurious” holons produce a chiral structure, due to , but the bands of “physical” holons produce an opposite chiral structure, due to . The induced additional Chern-Simons terms change, however, the braid statistics of the low-energy holon quasi-particle excitations (in Landau’s sense) near the ground state of the semionic holon liquid. Since the coefficients of the total, original plus induced, Chern-Simon actions for and are -1 and +1, respectively, we expect that the statistics of such quasi-particles is fermionic, as indeed suggested by preliminary calculations based on an approximate explicit expression for the low-energy behaviour of the holon Green function that will be presented in a separate paper. This change of statistics from the fields to the ”Landau” quasi-particle excitations is somewhat analogous to what happens in the composite fermion theory of the Fractional quantum Hall effect jain , where the quasi-particle excitations near the composite fermion ground state are anyons.
Above we discussed the situation in the PG “phase”, now we add a brief comment for the SM “phase”. As quoted in Sect. 2, the optimal spinon configuration , around which we expand the spinon fluctuations described by , acquires for hopping holons -flux phase factors in the SM “phase” that cancel the original -flux phase factors. The spinon coupling occurs only for the upper band and this additional phase factor modifies the dispersion of the upper band so that close to the Fermi surface it is turned into that of the - model in the tight-binding approximation; both compressibility and the Hall conductivity of the upper band still vanish. Since the lower band is not involved in the modification its Hall conductivity remains , hence even in SM phase the hopping holons have exclusion statistics 1/2.
On the basis of the result on the Fermi surface discussed in Sect. III and the generalization of the Luttinger theorem discussed in Ref. sent, , we suspect that the physical hole system, at least in the PG “phase” , possesses a topological order of the kind considered in the above quoted referencessent .
IV Conclusions
Let’s summarize our results. The Gutzwiller projection and the low dimensionality (1 or 2D), allow a gauging of the -charge and -spin symmetries of the - model leaving its physics completely unmodified. As a result at the lattice level the charge degrees of freedom, described by spinless holons, and the spin degrees of freedom, described by spinons, of the - model acquire a semionic braid statistics both in 2D, and in 1D, where this statistics holds also for the corresponding low-energy ”quasi-particles” and can be explicitly checked comparing with the exact solution. The additional freedom provided by the gauging allows a better simultaneous optimization of both and terms, and in 2D it introduces a novel kind of excitations, , the AF spin vortices. These are quantum distortions of the AF spin background in the subgroup of the -spin group unbroken by antiferromagnetism. Their cores are located on the empty sites of the 2D - model, mimicking the Zhang-Rice singlets of cuprates, and they record in their vorticity the Néel structure of the lattice. In a mean-field treatment at large scales their interaction with the spin degrees of freedom turn the long-range AF order of the model at half-filling into a short-range AF order above a critical doping and this implies a relaxation of the Gutzwiller constraint at large scales. Although with the Gutzwiller projection exactly implemented the charge degrees of freedom have physical bands empty at half-filling, at mean field level the constraint is relaxed and “spurious” filled lower holon bands appear, describing the unprojected holes at half-filling. With a proper regularization, the role of these “spurious” holon bands is to give an approximate but self-consistent description of the Gutzwiller projection on holons, providing an effective “vacuum” in which the “physical” hopping holons move. But this “vacuum” is topologically non-trivial, as shown by its non-vanishing Chern number or Hall conductivity, and this non-triviality deeply affects the “physical” upper bands, in particular forcing a 1/2 exclusion statistics for their semionic holons, as in 1D. The slave-particle gauge attraction between holon and spinon then produces a Fermi surface for holes, as holon-spinon low-energy bound states, with the addition of a -term, approximately consistent with the ARPES experiments in hole-doped cuprates mysy .As in 1D the parity and time-reversal symmetry are broken separately for the holon and spinon subsystems, due to their semionic nature, but for physical slave-particle gauge-invariant quantities they are restored.
To conclude, we remark that the spin-charge gauge approach allows to recover, sometimes even semi-quantitatively, many unusual experimental features of hole-doped cuprates, and for completeness we now briefly mention the most relevant results. We believe that the most interesting feature of the approach is that holes are composites made of only weakly bound holons and spinons, so that some physical responses are dominated by the spin carriers, in totally non-Fermi liquid manner. As noticed above, previously this approach was implemented in the approximation in which the 1/2 Haldane statistics for the holon was assumed, but, somewhat inconsistently, its semionic nature was not taken into account, consistently neglecting, however, the influence of AF spin vortices on holon hopping. The expected fermionic nature of the ”Landau” holon quasi-particle discussed in the previous section nevertheless suggests that the approximation made was already not unreasonable. Anyway a careful account of the two neglected effects mentioned above cannot change significantly the physical responses dominated by spinons, which are responsible for results that we now sketch in words, referring to the original papers for explicit formulas and plots.
A phenomenon naturally explained by this approach is the metal-insulator crossover (MIC) found decreasing in the in-plane resistivity of underdoped cuprates (see Refs. MIC, ). Although it is often attributed to disorder-induced localization, that interpretation is at odds with the fact that, depending on materials and dopings, MIC occurs from far below to far above the Ioffe-Regel limit. That interpretation is also at odds with the existence in a large range of temperatures, including the MIC, of a universal curveunir for a normalized resistivity as a function of , where can be identified as an inflection point in the in-plane resistivity. For these reasons we believe that the MIC is intrinsic, although disorder-induced localization may play a role at lower temperatures where, in fact, universality breaks down. In the spin-charge gauge approach the MIC can be easily explained: Due to the slave-particle gauge string binding spinon to holon, the velocity of the hole bound state is determined by the slowest among spinon and holon (Ioffe-Larkin rule il ). The holon has a metallic behavior with a FS, whereas, due to the AF gap, at low the spinon can only move by thermal diffusion leading to a semiconducting behavior. However, at higher temperatures its dynamics is dominated by the dissipation growing with induced by slave-particle gauge fluctuations, leading to a metallic behaviour. The universality is explained by the spinon dominance msy , leading to insensitivity to details of the FS, and even quantitatively the universal curve can be well reproduced mb . We call the low-pseudogap temperature at which the resistivity curve exhibits an inflection point and, on the basis of the comparison between the experimental and the theoretically derived resistivity curve, we identify it with the crossover from PG to SM in our approach. A similar crossover with increasing from a AF-gap dominated region to a gauge-induced dissipation dominated region can explain the peak in the spin-lattice relaxation rate in underdoped cuprates slr .
The spin-charge gauge approach provides a three-step mechanism for superconductivity that might explain several crossovers appearing in the phase-diagram of cuprates.
Firstly, at a temperature that we denote by , the attraction mediated by the AF-spin vortices described in Eq. (II.8) produces charge-pairing, the spin degrees of freedom being still unpaired. Since the formation of charge-pairs induces a reduction of the spectral weight on the FS of holons, inherited then by holes, we identify in cuprates as the temperature below which a pseudogap appears in the spectral weight of the hole (even well above in the -- model mg ), and we call this temperature high-pseudogap. Qualitatively many features of this high-pseudogap in the hole spectral weight derived in Ref. mg, are consistent with experimental data, but, according to the result of the present paper the influence of the semionic nature of the holon field should be reconsidered.
At a lower temperature, , the slave-particle gauge attraction between holon and spinon induces the formation of short-range spin-singlet (RVB) spinon pairs, in a sense, using the holon-pairs as the source of attraction, thus leading to a finite density of incoherent hole pairs. Comparing the behavior of spinon-pair density mfsy ,m with the intensity of the Nernst signal ner seen in cuprates, we identify this crossover as the onset of the diamagnetic/Nernst signals induced by magnetic vortices.
Finally, at an even lower temperature, the superconducting transition temperature , the hole pairs become coherent and a -wave hole condensate appears, leading to superconductivity. The presence of three crossover temperatures is typical of this approach and finds a reasonable correspondence in the experimental phase diagram of cupratesm .
In particular, for the same reason given for in-plane resistivity, the superfluid density satisfies Ioffe-Larkin rule and is dominated by spinons in the underdoped region. Below the low-energy effective action obtained integrating out the massive spinons is a Maxwell-gauged 3D XY model, where the angle-field of the XY model is the phase of the long-wave limit of the hole-pair field and the gauge field is the slave-particle gauge field.This explains the 3DXY critical exponent of the superfluid density found in experiments. Furthermore, as in the case of resistivity, the spinon dominance explains the experimental observation of a universal curve for the normalized superfluid density as a function of unis , which can be well reproduced even quantitatively by the spin-charge gauge approachmb .
Let us end this paper by remarking that we are computing some physical response dominated by holons, to check the effect of the semionic nature of the holon field in our approach, in comparison with the experimental data of cuprates. Preliminary calculations suggest that the main effect w.r.t. the previous approximate treatment is a modification of the wave-function renormalization constant of the hole, which becomes temperature independent allowing, for example, a recovery of the experimentally observed Fermi-liquid behaviour of the Knight shift at high in the ”strange-metal phase” of hole-doped cuprates (see e.g. Ref. sli, ).
Acknowledgements
We thank the Referees for stimulating comments that partially motivated the preparation of Ref. mysy, . F.Y. is supported by National Nature Science Foundation of China 11774143, and JCYJ20160531190535310. P.A.M. acknowledges the partial support from the Ministero Istruzione Universitá Ricerca (PRIN Project ”Collective Quantum Phenomena: From Strongly-Correlated Systems to Quantum Simulators”).
V Appendix
In this Appendix we outline the calculation of the Chern-Simons term for the upper band of holons in one of the Dirac double-cones. For simplicity we consider only the coupling to , the coupling with can be done in a similar way. The two terms don’t mix due to the factor in the -coupling arising from the fact that the two components of the Dirac field arise from different Néel sublattices, hence with opposite charge for . Following Ref. re, we consider a coupling to a field of constant field strength , calculate the expectation of the induced current
[TABLE]
with the gauge invariantly regularized Green function in the presence of , and we keep only the term proportional to . Its coefficient, which we denote by , multiplied by is the coefficient of the Chern-Simons action. We define and consider the case . According to the discussion in sect. III D, the Green functions for free ”physical” holons in momentum space is given by
[TABLE]
with . Then, using Schwinger’s proper time formalism, the Green function for the ”physical” holons in the limit can be represented as:
[TABLE]
The relevant term for the Chern-Simons action in is given by . Inserting this term in (V.1),(V) and performing the integral over spatial momenta one finds
[TABLE]
where denotes the principal value. In the limit the imaginary term disappears and one recovers the result . A similar calculation can be done for the band of ”spurious” holons with free Green function defined, as discussed in sect. III D, by
[TABLE]
Analogously one obtains, besides an imaginary term vanishing in the limit ,
[TABLE]
proving that indeed the lower band of ”spurious” holons has the Hall conductance calculated in sec. IIIC.
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