Peak Effect in Ca$_3$Rh$_4$Sn$_{13}$ : Vortex Phase Diagram and Evidences for Stepwise Amorphization of Flux Line Lattice

TL;DR

This study investigates the peak effect in Ca$_3$Rh$_4$Sn$_{13}$, revealing a stepwise fracturing of the flux line lattice and evidence for amorphization, leading to a detailed vortex phase diagram.

Contribution

It introduces a novel interpretation of the peak effect involving stepwise amorphization of the flux line lattice, contrasting with previous GFFLO-based explanations.

Findings

Discontinuous first order-like transitions in PE region

Path dependence of critical current density J_c(H,T)

Complete amorphization of FLL at (T_p, H_p) line

Abstract

The Peak Effect (PE) regime in a single crystal of Ca$_3$Rh$_4$Sn$_{13}$ has been investigated in detail via ac susceptibility as well as dc magnetization measurements. The PE region comprises two discontinuous first order like transitions, located near its onset and peak positions and reflects a stepwise fracturing of the flux line lattice (FLL). This scenario can be construed as an alternative to a scheme involving the appearance of Generalized Fulde-Ferrel-Larkin-Ovchinnikov (GFFLO) state as considered in the case of PE phenomenon in isostructural Yb$_3$Rh$_4$Sn$_{13}$ system. The procedure of thermal cycling across the onset position of PE produces an open hysteresis loop, which is consistent with the notion of the fracturing of the FLL. A study of thermomagnetic history dependence of different metastable vortex states shows the path dependence in the critical current density J_c(H,T) over a large part of the (H,T) parameter space. The path dependence in J_c ceases above the peak position of the PE, suggesting a complete amorphization and the loss of long range correlations of the FLL at (T_p, H_p) line. A plausible vortex phase diagram has been illustrated for Ca$_3$Rh$_4$Sn$_{13}$n and phases like an elastic solid, a plastic solid, a pinned amorphous and an unpinned amorphous states have been identified.