Spin dynamics in hole-doped two-dimensional S=1/2 Heisenberg antiferromagnets: ^{63}Cu NQR relaxation in La_{2-x}Sr_xCuO_4 for $x\leq 0.04$

TL;DR

This study investigates how hole doping affects spin dynamics in La_{2-x}Sr_xCuO_4 using ^{63}Cu NQR relaxation measurements, revealing persistent classical spin behavior and possible stripe formation at high temperatures.

Contribution

It provides new insights into the impact of low-level hole doping on spin correlations and the potential formation of stripe phases in La_{2-x}Sr_xCuO_4.

Findings

Spin stiffness constant decreases with doping but levels off beyond x=0.02.

High-temperature spin behavior remains in the renormalized classical regime.

Evidence suggests formation of microsegregated hole stripes.

Abstract

The effects on the correlated Cu^{2+} S = 1/2 spin dynamics in the paramagnetic phase of La_{2-x}Sr_xCuO_4 (for $x \lesssim 0.04$) due to the injection of holes are studied by means of ^{63}Cu NQR spin-lattice relaxation time T_1 measurements. The results are discussed in the framework of the connection between T_1 and the in-plane magnetic correlation length $\xi_{2D}(x,T)$. It is found that at high temperatures the system remains in the renormalized classical regime, with a spin stiffness constant $\rho_s(x)$ reduced by small doping to an extent larger than the one due to Zn doping. For $x\gtrsim 0.02$ the effect of doping on $\rho_s(x)$ appears to level off. The values for $\rho_s(x)$ derived from T_1 for $T\gtrsim 500$ K are much larger than the ones estimated from the temperature behavior of sublattice magnetization in the ordered phase ($T\leq T_N$). It is argued that these features are consistent with the hypothesis of formation of stripes of microsegregated holes.