Magnetoresistance of Granular Ferromagnets - Observation of a Magnetic Proximity Effect?

TL;DR

This study investigates how non-magnetic overlayers influence the magnetic and magnetoresistive properties of granular Ni films, revealing a possible magnetic proximity effect that induces ferromagnetic moments in the non-magnetic medium.

Contribution

It provides experimental evidence of a magnetic proximity effect in granular ferromagnets, linking inter-grain magnetic coupling to the magnetic susceptibility of overlayers.

Findings

Transition from superparamagnetic to ferromagnetic behavior observed.

Hysteresis in magnetoresistance develops with different overlayers.

Magnetic coupling correlates with the susceptibility of the overlayer material.

Abstract

We have observed a superparamagnetic to ferromagnetic transition in films of isolated Ni grains covered by non-magnetic overlayers. The magnetoresistance (MR) of the films was measured as a function of the overlayer thickness. Initially, the granular Ni films exhibited negative MR curves peaked at H=0. As different materials were deposited onto the grains hysteresis developed in the MR. This behavior is ascribed to an increase of the typical domain size due to magnetic coupling between grains. The strength of the inter-grain coupling is found to correlate with the magnetic susceptibility of the overlayer material. We discuss possible mechanisms for this coupling and suggest that the data may reflect the existence of a magnetic proximity effect (analogous to the well-known effect in superconductivity) in which a ferromagnetic moment is induced in the metallic non-magnetic medium.