Fluctuation-induced phase in CsCuCl3 in transverse magnetic field: Theory

TL;DR

This paper develops a Landau theory to explain fluctuation-induced incommensurate phases in CsCuCl3 under transverse magnetic fields, aligning theoretical predictions with recent experimental observations near the Neel temperature.

Contribution

It introduces a minimal Landau model incorporating fluctuation effects via a biquadratic term to explain new incommensurate phases in CsCuCl3.

Findings

Two incommensurate phases identified by the theory.

Qualitative agreement with experimental phase near T_N.

Fluctuations crucially influence the phase behavior.

Abstract

CsCuCl3 is a quantum triangular antiferromagnet, ferromagnetically stacked, with an incommensurate (IC) structure due to a Dzyaloshinskii-Moriya interaction. Because of the classical degeneracy caused by the frustration, fluctuations in CsCuCl3 have extraordinarily large effects, such as the phase transition in longitudinal magnetic field (normal to the planes, parallel to the IC wavenumber q) and the plateau in q in transverse field (perpendicular to q). We argue that fluctuations are responsible also for the new IC phase discovered in transverse field near the Neel temperature T_N, by T. Werner et al. [Solid State Commun. 102, p.609 (1997)]. We develop and analyse the corresponding minimal Landau theory; the effects of fluctuations on the frustration are included phenomenologically, by means of a biquadratic term. The Landau theory gives two IC phases, one familiar from previous studies; properties of the new IC phase, which occupies a pocket of the temperature-field phase diagram near T_N, agree qualitatively with those of the new phase found experimentally.