Electronic Raman-scattering study of low-energy excitations in single and double CuO_2-layer Tl-Ba-(Ca)-Cu-O superconductors

TL;DR

This study uses electronic Raman scattering to compare low-energy excitations in single and double CuO_2-layer Tl-Ba-(Ca)-Cu-O superconductors, revealing differences in gap ratios and screening effects.

Contribution

It provides the first detailed comparison of Raman spectra between single and double-layer Tl-based cuprate superconductors, highlighting differences in gap ratios and Coulomb screening.

Findings

Larger 2Δ/kBTc ratios in Tl-2212 than Tl-2201.

Stronger Coulomb screening in Tl-2201.

Similar coupling mechanisms for 2Δ-peak and continuum in both materials.

Abstract

Low energy Raman continuum and the redistribution of the continuum to a peak (2\Delta-peak) in the superconducting state have been studied in Tl-Ba-(Ca)-Cu-O superconductors with single (Tl-2201) and double (Tl-2212) CuO_2 layer. The 2\Delta/k_BT_c ratios in A_1g and B_1g symmetries are larger for Tl-2212 than for Tl-2201. The B_1g/A_1g gap ratio is also larger in Tl-2212. The A_1g intensities of the continuum and the 2\Delta-peak are significantly weaker than the B_1g intensities in Tl-2201, but are comparable in Tl-2212. This shows that the Coulomb screening is much stronger in Tl-2201. The change from Tl-2201 to Tl-2212 of the normalized A_1g 2\Delta-peak intensity is identical within experimental error to that of normalized A_1g continuum intensity. This suggests that the excitations forming the 2\Delta-peak and the continuum couple to light by the same mechanism.