Why Are Large Persistent Currents Observed in Small Gold Rings?

TL;DR

This paper uses computer simulations to show that simple non-interacting electron models with grain boundary scattering can produce large persistent currents in small gold rings, aligning with experimental observations.

Contribution

It demonstrates that grain boundary scattering models can explain large persistent currents in gold rings, contrasting with impurity scattering models.

Findings

Persistent currents coexist with small conductances in grain boundary models.

Different defect structures influence persistent currents and transport differently.

Proposes experiments to test the grain boundary explanation.

Abstract

It is demonstrated using three-dimensional computer simulations that some simple non-interacting electron models that include electron scattering by grain boundaries, exhibit coexistence of large persistent currents and small conductances, similar to that observed experimentally in isolated micron-scale gold rings. Models with simple grain boundaries, and models with small numbers of regularly stepped or atomically rough dilute grain boundaries have been studied and found to yield similar results, which differ markedly, however, from the predictions of models that assume only random impurity scattering. This difference is due to the fact that equilibrium persistent currents and non-equilibrium transport coefficients are physically different things and depend in different ways on the topology of the defect structure in a conducting ring. Experiments on metal and semiconductor rings that should be able to determine whether this is the explanation of the effects observed by Chandrasekhar et al. (Phys. Rev. Lett. 67, 3578 (1991)) are proposed.