Low temperature specific heat and possible gap to magnetic excitations in the Heisenberg pyrochlore antiferromagnet Gd2Sn207

TL;DR

This paper investigates the low-temperature specific heat of Gd2Sn2O7, proposing that its excitations are gapped magnons rather than gapless spin waves, challenging previous interpretations of anomalous T-squared behavior.

Contribution

It introduces a model showing that the low-energy excitations in Gd2Sn2O7 are gapped magnons, not gapless spin waves, explaining the observed specific heat behavior.

Findings

Gapped magnon excitations dominate low-temperature behavior.

T-squared specific heat arises from crossover to activated magnon regime.

Further measurements below 100 mK are needed to confirm the excitation spectrum.

Abstract

The Gd2Sn2O7 pyrochlore Heisenberg antiferromagnet displays a phase transition to a four sublattice Neel ordered state at a temperature near 1 K. Despite the seemingly conventional nature of the ordered state, the specific heat has been found to be described in the temperature range 350-800 mK by an anomalous T-squared power law. A similar temperature dependence has also been reported for Gd2Ti2O7, another pyrochlore Heisenberg material. Such anomalous T-squared behavior in Cv has been argued to be correlated to an unusual energy-dependence of the density of states which also seemingly manifests itself in low-temperature spin fluctuations found in muon spin relaxation experiments. In this paper, we report calculations of Cv that consider spin wave like excitations out of the Neel order observed in Gd2Sn2O7 and argue that the parametric T-squared behavior does not reflect the true low-energy excitations of Gd2Sn2O7. Rather, we find that the low-energy excitations of this material are antiferromagnetic magnons gapped by single-ion and dipolar anisotropy effects, and that the lowest temperature of 350 mK considered in previous specific heat measurements accidentally happens to coincide with a crossover temperature below which magnons become thermally activated and Cv takes an exponential form. We argue that further specific heat measurements that extend down to at least 100 mK are required in order to ascribe an unconventional description of magnetic excitations out of the ground state of Gd2Sn2O7 or to invalidate the standard picture of gapped excitations proposed herein.