Anomalous physical properties of underdoped weak-ferromagnetic superconductor RuSr$_2$EuCu$_{2}$O$_{8}$

TL;DR

This study investigates the unusual magnetic and superconducting behaviors of underdoped RuSr$_2$EuCu$_2$O$_8$, revealing a spontaneous vortex state, vortex liquid region, and magnetic entropy consistent with Gd$^{3+}$ ordering, highlighting complex interplay between magnetism and superconductivity.

Contribution

The paper provides detailed experimental insights into the coexistence and interplay of weak ferromagnetism and superconductivity in underdoped RuSr$_2$EuCu$_2$O$_8$, including vortex dynamics and magnetic entropy analysis.

Findings

Existence of spontaneous vortex state between 16 K and 36 K.

Identification of vortex melting transition at 21 K.

Confirmation of Gd$^{3+}$ magnetic entropy near expected value.

Abstract

Similar to the optimal-doped, weak-ferromagnetic (WFM induced by canted antiferromagnetism, T$_{Curie}$ = 131 K) and superconducting (T$_{c}$ = 56 K) RuSr$_{2}$GdCu$_{2}$O$_{8}$, the underdoped RuSr$_{2}$EuCu$_{2}$O$_{8}$ (T$_{Curie}$ = 133 K, T$_{c}$ = 36 K) also exhibited a spontaneous vortex state (SVS) between 16 K and 36 K. The low field ($\pm$20 G) superconducting hysteresis loop indicates a weak and narrow Meissner state region of average lower critical field B$_{c1}^{ave}$(T) = B$_{c1}^{ave}$(0)[1 - (T/T$_{SVS}$)$^{2}$], with B$_{c1}^{ave}$(0) = 7 G and T$_{SVS}$ = 16 K. The vortex melting transition (T$_{melting}$ = 21 K) below T$_{c}$ obtained from the broad resistivity drop and the onset of diamagnetic signal indicates a vortex liquid region due to the coexistence and interplay between superconductivity and WFM order. No visible jump in specific heat was observed near T$_{c}$ for Eu- and Gd-compound. This is not surprising, since the electronic specific heat is easily overshadowed by the large phonon and weak-ferromagnetic contributions. Furthermore, a broad resistivity transition due to low vortex melting temperature would also lead to a correspondingly reduced height of any specific heat jump. Finally, with the baseline from the nonmagnetic Eu-compound, specific heat data analysis confirms the magnetic entropy associated with antiferromagnetic ordering of Gd$^{3+}$ (J = S = 7/2) at 2.5 K to be close to $\it{N_{A}k}$ ln8 as expected.