Exchange energy and generalized polarization in the presence of spin-orbit coupling in two dimensions
S. Chesi, G. F. Giuliani

TL;DR
This paper develops a generalized framework for exchange energy in two-dimensional electron systems with spin-orbit coupling, revealing that polarization does not always increase exchange energy, which aligns with recent experimental observations.
Contribution
It introduces a new formulation of exchange energy using generalized fractional polarization, highlighting its impact on spin states in 2D systems with spin-orbit interaction.
Findings
Generalized polarization does not necessarily increase exchange energy.
Unpolarized states can be energetically favored due to spin-orbit effects.
Results qualitatively match recent experimental findings.
Abstract
We discuss a general form of the exchange energy for a homogeneous system of interacting electrons in two spatial dimensions which is particularly suited in the presence of a generic spin-orbit interaction. The theory is best formulated in terms of a generalized fractional electronic polarization. Remarkably we find that a net generalized polarization does not necessarily translate into an increase in the magnitude of the exchange energy, a fact that in turn favors unpolarized states. Our results account qualitatively for the findings of recent experimental investigations.
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Taxonomy
TopicsQuantum and electron transport phenomena · Advanced Chemical Physics Studies · Molecular Junctions and Nanostructures
