What makes a crystal supersolid ?

TL;DR

This paper reviews the longstanding mystery of supersolidity, discusses recent experimental findings in helium-4, and explores alternative scenarios and fundamental questions about the conditions needed for a true supersolid phase.

Contribution

It critically examines experimental data on helium-4, evaluates alternative mechanisms for supersolidity, and discusses the theoretical challenges in realizing an ideal supersolid.

Findings

Experimental evidence suggests superfluid-like response in solid He-4.

Homogeneous supersolid phase remains unconfirmed and controversial.

Alternative scenarios involve defects and metastable phases.

Abstract

For nearly half a century the supersolid phase of matter has remained mysterious, not only eluding experimental observation, but also generating a great deal of controversy among theorists. Recent discovery of what is interpreted as a non-classical moment of inertia at low temperature in solid He-4 has elicited much excitement as a possible first observation of a supersolid phase. In the two years following the discovery, however, more puzzles than answers have been provided to the fundamental issue of whether the supersolid phase exists, in helium or any other naturally occurring condensed matter system. Presently, there is no established theoretical framework to understand the body of experimental data on He-4. Different microscopic mechanisms that have been suggested to underlie superfluidity in a perfect quantum crystal do not seem viable for \he4, for which a wealth of experimental and theoretical evidence points to an insulating crystalline ground state. This perspective addresses some of the outstanding problems with the interpretation of recent experimental observations of the apparent superfluid response in He-4 (seen now by several groups) and discusses various scenarios alternative to the homogeneous supersolid phase, such as superfluidity induced by extended defects of the crystalline structure which include grain boundaries, dislocations, anisotropic stresses, etc. Can a metastable superfluid "glassy" phase exist, and can it be relevant to some of the experimental observations ? One of the most interesting and unsolved fundamental questions is what interatomic potentials, given the freedom to design one, can support an ideal supersolid phase in continuous space, and can they be found in Nature.