Magnetic excitations in multiferroic TbMnO3

TL;DR

This study investigates magnetic excitations in multiferroic TbMnO3 using inelastic neutron scattering, revealing low-energy magnons associated with spiral and sinusoidal magnetic phases, and identifying modes that couple to electric polarization.

Contribution

It provides a detailed characterization of magnon modes in TbMnO3, including their polarization and coupling to electric polarization, supported by neutron-polarization analysis and infrared spectroscopy.

Findings

Identified three low-lying magnon modes at the incommensurate zone center.

The lowest mode is a sliding mode of the spiral.

The 2.5 meV mode is a hybridized phonon-magnon excitation.

Abstract

The magnetic excitations in multiferroic TbMnO3 have been studied by inelastic neutron scattering in the spiral and sinusoidally ordered phases. At the incommensurate magnetic zone center of the spiral phase, we find three low-lying magnons whose character has been fully determined using neutron-polarization analysis. The excitation at the lowest energy is the sliding mode of the spiral, and two modes at 1.1 and 2.5meV correspond to rotations of the spiral rotation plane. These latter modes are expected to couple to the electric polarization. The 2.5meV-mode is in perfect agreement with recent infra-red-spectroscopy data giving strong support to its interpretation as an hybridized phonon-magnon excitation.