Interplay of electron-lattice interactions and superconductivity in Bi2Sr2CaCu2O8+d

TL;DR

This study uses advanced scanning tunnelling microscopy to image bosonic modes in a high-Tc superconductor, revealing local lattice vibrations that interact with superconductivity and are unaffected by electronic or magnetic changes.

Contribution

It provides direct atomic-scale imaging of bosonic modes in Bi2Sr2CaCu2O8+d, identifying them as lattice vibrations and showing their spatial anticorrelation with superconducting gaps.

Findings

Bosonic modes are spatially heterogeneous at the nanometre scale.

Isotope substitution shifts the mode energies, confirming lattice vibrations.

Modes are anticorrelated with superconducting gap energies.

Abstract

Formation of electron pairs is essential to superconductivity. For conventional superconductors, tunnelling spectroscopy has established that pairing is mediated by bosonic modes (phonons); a peak in the second derivative of tunnel current d2I/dV2 corresponds to each phonon mode . For high-transition-temperature (high-Tc) superconductivity, however, no boson mediating electron pairing has been identified. One explanation could be that electron pair formation and related electron-boson interactions are heterogeneous at the atomic scale and therefore challenging to characterize. However, with the latest advances in d2I/dV2 spectroscopy using scanning tunnelling microscopy, it has become possible to study bosonic modes directly at the atomic scale . Here we report d2I/dV2 imaging studies of the high-Tc superconductor Bi2Sr2CaCu2O8+d. We find intense disorder of electron-boson interaction energies at the nanometre scale, along with the expected modulations in d2I/dV2 (refs 9,10). Changing the density of holes has minimal effects on both the average mode energies and the modulations, indicating that the bosonic modes are unrelated to electronic or magnetic structure. Instead, the modes appear to be local lattice vibrations, as substitution of 18O for 16O throughout the material reduces the average mode energy by approximately 6 per cent - the expected effect of this isotope substitution on lattice vibration frequencies. Significantly, the mode energies are always spatially anticorrelated with the superconducting pairing-gap energies, suggesting an interplay between these lattice vibration modes and the superconductivity.