Anomalous Hall Effect in three ferromagnets: EuFe4Sb12, Yb14MnSb11, and Eu8Ga16Ge30

TL;DR

This study investigates the anomalous Hall effect in three ferromagnetic Zintl compounds, revealing that the intrinsic Hall conductivity is a temperature-independent ground state property consistent with recent theoretical models.

Contribution

It provides experimental measurements of the anomalous Hall conductivity in three ferromagnets, supporting theories that intrinsic Hall conductivity is a fundamental ground state property.

Findings

Intrinsic Hall conductivity is temperature-independent below Tc.

Measured Hall conductivities are consistent with theoretical predictions.

Low carrier concentrations enable clear separation of anomalous and normal Hall effects.

Abstract

The Hall resistivity (Rho_xy), resistivity (Rho_xx), and magnetization of three metallic ferromagnets are investigated as a function of magnetic field and temperature. The three ferromagnets, EuFe4Sb12 (Tc = 84 K), Yb14MnSb11 (Tc = 53 K), and Eu8Ga16Ge30 (Tc = 36 K) are Zintl compounds with carrier concentrations between 1 x 10^21 cm^-3 and 3.5 x 10^21 cm^-3. The relative decrease in Rho_xx below Tc [Rho_xx(Tc)/Rho_xx(2 K)] is 28, 6.5, and 1.3 for EuFe4Sb12, Yb14MnSb11, and Eu8Ga16Ge30 respectively. The low carrier concentrations coupled with low magnetic anisotropies allow a relatively clean separation between the anomalous (Rho_'xy), and normal contributions to the measured Hall resistivity. For each compound the anomalous contribution in the zero field limit is fit to alpha Rho_xx + sigma_xy rho_xx^2 for temperatures T < Tc. The anomalous Hall conductivity, sigma_xy, is -220 +- 5 (Ohm^-1 cm^-1), -14.7 +- 1 (Ohm^-1 cm^-1), and 28 +- 3 (Ohm^-1 cm^-1) for EuFe4Sb12, Yb14MnSb11, and Eu8Ga16Ge30 respectively and is independent of temperature for T < Tc if the change in spontaneous magnetization (order parameter) with temperature is taken into account. These data are consistent with recent theories of the anomalous Hall effect that suggest that even for stochiometric ferromagnetic crystals, such as those studied in this article, the intrinsic Hall conductivity is finite at T = 0, and is a ground state property that can be calculated from the electronic structure.