Magnetization dynamics in dysprosium orthoferrites via inverse Faraday effect

TL;DR

This paper investigates the ultrafast magnetization dynamics in dysprosium orthoferrites induced by the inverse Faraday effect using a combined experimental and theoretical approach, revealing mode excitations and decay mechanisms.

Contribution

It presents a theoretical model based on free energy and Landau-Lifshitz-Gilbert equations that explains experimental observations of laser-induced magnetization dynamics in orthoferrites.

Findings

Single resonance mode excited along z-axis

Magnon-magnon scattering affects decay on picosecond scale

Different modes excited with x-axis field pulse

Abstract

The ultrafast non-thermal control of magnetization has recently become feasible in canted antiferromagnets through photomagnetic instantaneous pulses [A.V. Kimel {\it et al.}, Nature {\bf 435}, 655 (2005)]. In this experiment circularly polarized femtosecond laser pulses set up a strong magnetic field along the wave vector of the radiation through the inverse Faraday effect, thereby exciting non-thermally the spin dynamics of dysprosium orthoferrites. A theoretical study is performed by using a model for orthoferrites based on a general form of free energy whose parameters are extracted from experimental measurements. The magnetization dynamics is described by solving coupled sublattice Landau-Lifshitz-Gilbert equations whose damping term is associated with the scattering rate due to magnon-magnon interaction. Due to the inverse Faraday effect and the non-thermal excitation, the effect of the laser is simulated by magnetic field Gaussian pulses with temporal width of the order of hundred femtoseconds. When the field is along the z-axis, a single resonance mode of the magnetization is excited. The amplitude of the magnetization and out-of-phase behavior of the oscillations for fields in z and -z directions are in good agreement with the cited experiment. The analysis of the effect of the temperature shows that magnon-magnon scattering mechanism affects the decay of the oscillations on the picosecond scale. Finally, when the field pulse is along the x-axis, another mode is excited, as observed in experiments. In this case the comparison between theoretical and experimental results shows some discrepancies whose origin is related to the role played by anisotropies in orthoferrites.