muSR study of the Cu-spin dynamics in the electron-doped high-Tc cuprate of Pr0.86LaCe0.14Cu1-y(Zn,Ni)yO4

TL;DR

This study investigates how Zn and Ni substitutions affect Cu-spin dynamics in electron-doped cuprates using muSR, revealing changes in magnetic order and spin fluctuation behavior at low temperatures.

Contribution

It provides new insights into the effects of Zn and Ni substitution on Cu-spin dynamics and magnetic ordering in electron-doped cuprates using muSR measurements.

Findings

Long-range antiferromagnetic order observed in as-grown samples.

Spin fluctuations slow down at low temperatures in reduced samples.

No significant difference between Zn and Ni effects on spin dynamics.

Abstract

Effects of the Zn- and Ni-substitution on the Cu-spin dynamics in the electron-doped Pr0.86LaCe0.14Cu1-y(Zn,Ni)yO4+a-d with y = 0, 0.01, 0.02, 0.05 and different values of the reduced oxygen content d have been studied using zero-field muon-spin-relaxation (muSR) measurements at temperatures down to 2 K. For the as-grown sample (d = 0, y = 0) and the sample with a very small d value (d < 0.01, y = 0), a muon-spin precession due to long-range antiferromagnetic order has been observed. On the other hand, no precession has been observed for moderately oxygen-reduced samples (0.01 < d < 0.09). It has been found that for all the samples of 0.01 < d < 0.09 the asymmetry A(t) (muSR time spectrum) in the long-time region increases with decreasing temperature at low temperatures, suggesting possible slowing-down of the Cu-spin fluctuations. On the other hand, no significant difference between Zn- and Ni-substitution effects on the slowing down of the Cu-spin fluctuations has been observed.