Unified Description of Aging and Rate Effects in Yield of Glassy Solids

TL;DR

This paper investigates how aging and deformation rate influence the shear yield stress of glassy solids, revealing a universal behavior through simulations and a phenomenological model.

Contribution

It introduces a unified phenomenological model that captures both aging and rate effects on yield stress in glassy materials, supported by molecular simulation data.

Findings

Yield stress increases logarithmically with age and rate.

A sharp transition in rate dependence occurs at a decreasing rate with age.

Data collapse onto a universal curve across temperatures.

Abstract

The competing effects of slow structural relaxations (aging) and deformation at constant strain rate on the shear yield stress $\tau^y$ of simple model glasses are examined using molecular simulations. At long times, aging leads to a logarithmic increase in density and $\tau^y$. The yield stress also rises logarithmically with rate, but shows a sharp transition in slope at a rate that decreases with increasing age. We present a simple phenomenological model that includes both intrinsic rate dependence and the change in properties with the total age of the system at yield. As predicted by the model, all data for each temperature collapse onto a universal curve.