Spontaneous decay dynamics in atomically doped carbon nanotubes

TL;DR

This paper investigates the non-exponential spontaneous decay of atoms near carbon nanotubes, revealing strong non-Markovian effects, vacuum-field Rabi oscillations, and controllable atom-field interactions for nanophotonics applications.

Contribution

It demonstrates the non-exponential decay dynamics and strong coupling effects of atoms near carbon nanotubes, highlighting control over atom-field interactions via atom-nanotube distance.

Findings

Non-exponential decay dynamics observed near carbon nanotubes

Vacuum-field Rabi oscillations indicate strong atom-field coupling

Decay behavior transitions from non-exponential to exponential with distance

Abstract

We report a strictly non-exponential spontaneous decay dynamics of an excited two-level atom placed inside or at different distances outside a carbon nanotube (CN). This is the result of strong non-Markovian memory effects arising from the rapid variation of the photonic density of states with frequency near the CN. The system exhibits vacuum-field Rabi oscillations, a principal signature of strong atom-vacuum-field coupling, when the atom is close enough to the nanotube surface and the atomic transition frequency is in the vicinity of the resonance of the photonic density of states. Caused by decreasing the atom-field coupling strength, the non-exponential decay dynamics gives place to the exponential one if the atom moves away from the CN surface. Thus, atom-field coupling and the character of the spontaneous decay dynamics, respectively, may be controlled by changing the distance between the atom and CN surface by means of a proper preparation of atomically doped CNs. This opens routes for new challenging nanophotonics applications of atomically doped CN systems as various sources of coherent light emitted by dopant atoms.