Analysis of resonant inelastic x-ray scattering in La2CuO4

TL;DR

This paper provides a theoretical explanation for RIXS spectra in La2CuO4, identifying key peaks and their origins, and emphasizes the importance of electron correlation in understanding the experimental observations.

Contribution

It offers a semiquantitative theoretical model that explains the characteristic peaks in RIXS spectra of La2CuO4, highlighting the role of electron correlation.

Findings

Two peaks attributed to charge transfer excitation match experimental data

The lowest energy peak shows significant dispersion (~0.8 eV)

Electron correlation is crucial for explaining the spectra's energy-momentum dependence

Abstract

We provide a semiquantitative explanation of a recent experiment on the resonant inelastic x-ray scattering (RIXS) in insulating cuprate La2CuO4 (Y.J. Kim et al., Phys. Rev. Lett. 89, 177003 (2002).). We show theoretically that there are three characteristic peaks in RIXS spectra, two of which are attributed to the charge transfer excitation and are reasonably assigned to those observed experimentally. The lowest energy peak has a relatively large dispersion ($\sim 0.8$ eV) and is suppressed near the zone corner (\pi, \pi), in agreement with the experiment. We stress that electron correlation is an essential factor for explaining the overall energy-momentum dependence of the RIXS spectra consistently.