Onset of antiferromagnetism in UPt_{3} via Th-substitution studied by muon spin spectroscopy

TL;DR

This study uses muon spin spectroscopy to investigate how Th substitution induces antiferromagnetism in UPt_{3}, revealing a gradual transition with disorder effects influencing magnetic fluctuations.

Contribution

It provides detailed experimental insights into the onset and nature of antiferromagnetism in Th-doped UPt_{3} using muon spin spectroscopy.

Findings

Weak magnetic signals appear at low Th content below 2 K.

Spontaneous oscillations indicate LMAF phase for 0.006 <= x <= 0.05.

Disorder broadens the magnetic transition and affects fluctuation dynamics.

Abstract

Muon spin spectroscopy has been used to study in detail the onset of large-moment antiferromagnetism (LMAF) in UPt_{3} as induced by Th substitution. Zero-field experiments have been carried out on a series of polycrystalline U_{1-x}Th_{x}Pt_{3} (0 <= x <= 0.05) samples in the temperature range 0.04 - 10 K. At low Th content (x <= 0.002) magnetic ordering on the time scale of the uSR experiment (10^{-8} s) is not detected. For x = 0.005 a weak magnetic signal appears below T = 2 K, while for 0.006 <= x <= 0.05, spontaneous oscillations in the uSR spectra signal the presence of the LMAF phase. The data are well described by a two-component depolarization function, combining the contribution of a polycrystalline antiferromagnet and a Kubo-Lorentzian response. However, the transition into the antiferromagnetic phase is quite broad. For x = 0.01 and 0.02, a weak magnetic signal appears below about 7 K, which is well above the mean-field transition temperatures. The broadening may be a result of the effects of disorder on the time fluctuations associated with anomalous small-moment antiferromagnetism.