Magneto-transport study of intra- and intergrain transitions in the magnetic superconductors RuSr2GdCu2O8 and RuSr2(Gd1.5Ce0.5)Cu2O10

TL;DR

This study investigates the magnetic and superconducting properties of RuSr2GdCu2O8 and RuSr2(Gd1.5Ce0.5)Cu2O10, revealing intra- and intergrain transitions, effects of magnetic fields, and the role of structural boundaries and layer separation.

Contribution

It provides a detailed analysis of intra- and intergrain superconducting transitions and their magnetic field dependence, highlighting the influence of structural and magnetic features in these compounds.

Findings

Intra- and intergrain peaks identified in resistance derivatives.

Intragrain transition temperature remains stable up to 0.1 T in Ru-(1212).

Intergrain transition amplitude increases sharply with magnetic field.

Abstract

A characterization of the magnetic superconductors RuSr2GdCu2O8 [Ru-(1212)] and RuSr2(Gd1.5Ce0.5)Cu2O10 [Ru-(1222)] through resistance measurements as a function of temperature and magnetic field is presented. Two peaks in the derivative of the resistive curves are identified as intra- and intergrain superconducting transitions. Strong intragrain granularity effects are observed, and explained by considering the antiphase boundaries between structural domains of coherently rotated RuO6 octahedra as intragrain Josephson-junctions. A different field dependence of the intragrain transition temperature in these compounds was found. For Ru-(1212) it remains unchanged up to 0.1 T, decreasing for higher fields. In Ru-(1222) it smoothly diminishes with the increase in field even for a value as low as 100 Oe. These results are interpreted as a consequence of a spin-flop transition of the Ru moments. The large separation between the RuO2 layers in Ru-(1222) promotes a weak interlayer coupling, leading the magnetic transition to occur at lower fields. The suppression rate of the intragrain transition temperature is about five times higher for Ru-(1222), a result we relate to an enhancement of the 2D character of the vortex structure. A distinctive difference with conventional cuprates is the sharp increase in amplitude of the intergrain peak in both systems, as the field is raised, which is ascribed to percolation through a fraction of high quality intergrain junctions.