Phase separation effects in charge-ordered Pr0.5Ca0.5MnO3 thin film

TL;DR

This study investigates phase separation in Pr0.5Ca0.5MnO3 thin films, revealing a ferromagnetic phase embedded within the charge-ordered phase, with properties influenced by magnetic field orientation and strength.

Contribution

It provides new insights into the magnetic anisotropy and phase coupling in Pr0.5Ca0.5MnO3 thin films using Electron Spin Resonance techniques.

Findings

Presence of a ferromagnetic phase within charge-ordered phase.

Ferromagnetic phase exhibits easy plane magnetic anisotropy.

Magnetic field orientation affects phase coupling and resonance behavior.

Abstract

Compressed Pr0.5Ca0.5MnO3 films (250nm) deposited on LaAlO3 have been studied by Electron Spin Resonance technique under high frequency and high magnetic field. We show evidences for the presence of a ferromagnetic phase (FM) embedded in the charge-order phase (CO), in form of thin layers which size depends on the strength and orientation of the magnetic field (parallel or perpendicular to the substrate plane). This FM phase presents an easy plane magnetic anisotropy with an anisotropy constant 100 times bigger than typical bulk values. When the magnetic field is applied perpendicular to the substrate plane, the FM phase is strongly coupled to the CO phase whereas for the parallel orientation it keeps an independent ferromagnetic resonance even when the CO phase becomes antiferromagnetic.