# On-Chip Plasmonic Slit-Cavity Platform for Room-Temperature Strong Coupling with Deterministically Positioned Colloidal Quantum Dots

**Authors:** Jin Qin, Benedikt Schurr, Patrick Pertsch, Daniel Friedrich, Max Knopf, Saeid Asgarnezhad-Zorgabad, Lars Meschede, Daniel D. A. Clarke, Monika Emmerling, Artur Podhorodecki, Ortwin Hess, Bert Hecht

PMC · DOI: 10.1021/acs.nanolett.5c05910 · Nano Letters · 2026-02-27

## TL;DR

Researchers developed a compact on-chip platform that enables strong coupling between quantum dots and plasmonic cavities at room temperature.

## Contribution

A deterministic fabrication method for plasmonic slit-cavities with colloidal quantum dots is introduced for room-temperature quantum technologies.

## Key findings

- Photoluminescence-resolved Rabi splitting was observed at room temperature in precharacterized plasmonic cavities.
- Device-to-device variations correlated with the average number of coupled quantum dots.
- Integration of electrodes enabled electrical tuning, though limited by spectral diffusion at room temperature.

## Abstract

Strong coupling between quantum emitters and optical
cavities underpins
many quantum photonic technologies, yet achieving this regime at room
temperature in compact, deterministic on-chip platforms remains challenging
due to the difficulty of fabricating cavities with ultrasmall mode
volumes and precisely positioning quantum emitters. Here, we demonstrate
a robust quantum plasmonic device in which colloidal quantum dots
are strongly coupled to plasmonic slit cavities. Our dielectrophoresis-based
positioning technique with real-time photoluminescence feedback enables
parallel device fabrication and straightforward integration with additional
optical elements, such as waveguides. Our measurements reveal clear
photoluminescence-resolved Rabi splitting at room temperature in precharacterized
cavities, with device-to-device variations scaling with the average
number of coupled quantum dots. While electrical tuning via the quantum-confined
Stark effect is enabled by integrated electrodes, its impact is largely
overshadowed by room-temperature spectral diffusion. These results
establish a scalable and electrically addressable plasmonic platform
for room-temperature quantum technologies.

## Full-text entities

- **Chemicals:** metal (MESH:D008670), water (MESH:D014867), TiN (MESH:D014001), helium (MESH:D006371), Si (MESH:D012825), silver (MESH:D012834), ZnS (MESH:D015032), Au (MESH:D006046), Ga (MESH:D005708), Au-Ag alloy (-)

## Full text

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## Figures

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## References

40 references — full list in the complete paper: https://tomesphere.com/paper/PMC13022876/full.md

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Source: https://tomesphere.com/paper/PMC13022876