# A Critical Comparison of Exposure Estimators for Airborne Particulate Matter in Urban Cyclists

**Authors:** Elie Al Marj, Ilann Mahou, Roy M. Harrison, Francis D. Pope, Alexandra Fort, Aurelie Charron

PMC · DOI: 10.3390/toxics14020179 · Toxics · 2026-02-17

## TL;DR

This study shows that using inhaled dose metrics, rather than average air pollution concentrations, better captures exposure differences among urban cyclists.

## Contribution

The study introduces and validates a simplified method for calculating inhaled doses during cycling, improving exposure classification accuracy.

## Key findings

- Simplified dose calculations closely matched full temporal integration methods (r > 0.999).
- Up to 50% of participants changed exposure categories when using dose-based metrics instead of average concentrations.
- Ultrafine particles showed the highest reclassification rate between exposure quartiles.

## Abstract

Urban cyclists experience elevated traffic-related air pollutant (TRAP) exposures due to proximity to emissions and increased breathing rates during exercise. Conventional assessments rely on concentration summaries, which may misrepresent actual inhaled doses and misclassify individuals in health studies. Street-level concentrations exhibit high temporal variability, producing non-normal distributions that challenge conventional averaging approaches. This study compares concentration- and dose-based methods to characterize cyclist exposure during urban commuting. Fifty-seven healthy adults completed cycling trips on two 9-km routes (high- and low-traffic) using conventional or electrically assisted bicycles. Real-time monitoring measured black carbon, ultrafine particles, PM2.5, and PM10. Heart rate-derived breathing rates enabled individualized inhaled dose calculations using three temporal integration methods. Mean concentrations correlated strongly with time-integrated concentrations (r = 0.988–0.998). Simplified dose calculations closely approximated full temporal integration (r > 0.999), with median dose ratios of 0.99–1.01. However, correlations between mean concentrations and inhaled doses were weaker (r = 0.72–0.78). Between 29% and 50% of participants changed exposure quartiles when comparing concentration- and dose-based classifications, with the highest reclassification for ultrafine particles (46–50%). These findings demonstrate that physiological variability substantially influences exposure classification during active commuting, supporting the integration of inhaled dose metrics in cyclist exposure assessment and epidemiological studies.

## Linked entities

- **Chemicals:** black carbon (PubChem CID 172866199)

## Full-text entities

- **Diseases:** cardiovascular or respiratory disorders (MESH:D018376), CTF (MESH:D005596), injury to (MESH:D014947), Ventilation (MESH:D053717), ATF (MESH:D001528)
- **Chemicals:** CB (-), carbon (MESH:D002244)
- **Species:** Homo sapiens (human, species) [taxon 9606]

## Full text

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## Figures

3 figures with captions in the complete paper: https://tomesphere.com/paper/PMC12945186/full.md

## References

58 references — full list in the complete paper: https://tomesphere.com/paper/PMC12945186/full.md

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Source: https://tomesphere.com/paper/PMC12945186