Thermal and filler concentration modulation of charge transport mechanism and dielectric properties in high-entropy oxide (CoCrFeNiMn)3O4-acrylic polymer composite
Samer I. Daradkeh, Ammar Alsoud, Tomáš Spusta, Vaclav Pouchlý, Alexandr Knápek, Pavel Tofel, Dinara Sobola
TL;DR
This study explores how temperature and filler concentration affect the electrical properties of acrylic polymer composites with a high-entropy oxide filler.
Contribution
The paper introduces a systematic analysis of HEO-polymer composites' dielectric behavior under varying temperature and filler concentration.
Findings
Filler concentration significantly enhances dielectric performance in HEO-polymer composites.
Temperature and HEO-850 concentration are key parameters governing the electrical behavior of the composites.
HEO's compositional complexity contributes to unique dielectric properties suitable for advanced applications.
Abstract
This study investigates the dielectric properties of polymer composites comprising an acrylic matrix and high-entropy oxide (HEO) (CoCrFeNiMn)3O4 filler. Single-phase HEO was synthesized via solid-state reaction followed by calcination at 850 °C (HEO-850). The research systematically examines the temperature- and concentration-dependent evolution of dielectric properties and charge transport mechanisms within these composite systems. Our findings reveal distinct correlations between filler concentration and dielectric performance enhancement. The unique properties of HEOs, stemming from their compositional complexity and structural characteristics, position these composite materials as promising candidates for advanced dielectric applications. The study elucidates fundamental parameters (temperature and filler concentration of HEO-850) governing the electrical behavior of HEO-polymer…
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Taxonomy
TopicsDielectric materials and actuators · Polymer Nanocomposite Synthesis and Irradiation · Dielectric properties of ceramics