# 3D Printed Flexible Piezoelectric Sensors for Integrated Hybrid Electronics

**Authors:** Daniel Wai Hou Ng, Hassene Ben Atitallah, Ghazaleh Haghiashtiani, Jinsheng Fan, Hyunjun Kim, Guebum Han, Riyan Mendonsa, Razman Zambri, Michael C. McAlpine

PMC · DOI: 10.1002/smll.202511146 · Small (Weinheim an Der Bergstrasse, Germany) · 2025-12-31

## TL;DR

Researchers developed a 3D printing method to create flexible piezoelectric sensors for wearable electronics and hybrid systems.

## Contribution

A direct-ink-writing 3D printing approach for high-performance flexible piezoelectric devices using PVDF-TrFE.

## Key findings

- Achieved a d31 coefficient of 12.70 ± 0.71 pC·N−1 in 3D printed PVDF-TrFE transducers.
- Fabricated three proof-of-concept devices including a tactile-sensing electronic skin and a hybrid system with quantum dot LEDs.

## Abstract

The ability to 3D print high performance smart materials and multifunctional devices, all seamlessly integrated via a common manufacturing platform, can yield advances in soft robotics, wearable electronics, and human‐machine interfaces. One of the most important smart materials in this context is piezoelectrics, due to their dual capabilities in sensing and actuating, which are critical for creating intelligent, responsive systems. In this study, we develop a direct‐ink‐writing (DIW) 3D printing approach for creating flexible and wearable piezoelectric devices using solution‐processed poly(vinylidene fluoride‐co‐trifluoroethylene) (PVDF‐TrFE) as the functional ink. Ferroelectric and actuation‐based characterizations are conducted to guide systematic optimization of the electrical poling conditions, yielding high performance 3D printed PVDF‐TrFE transducers with d31
 coefficient of 12.70 ± 0.71 pC·N−1. Three proof‐of‐concept smart devices were then fabricated: (1) a touch‐based wearable human‐machine interface for interactive gaming, (2) a tactile‐sensing “electronic skin,” and (3) a multifunctional hybrid electronic system combining piezoelectric sensors and quantum dot light‐emitting diodes, all fully 3D printed. This work comprehensively demonstrates the ability for 3D printing to generate high performance materials and devices, the use of 3D printing for wearable piezoelectric sensor fabrication, and the versatility of 3D printing for the seamless multifunctional integration of hybrid electronic systems.

A comprehensive 3D printing strategy can fabricate high performance piezoelectric transducers on various substrates for wearable and flexible electronics applications. Demonstrations include human‐machine interfaces, tactile electronic skin, and a multifunctional system integrating piezoelectric sensors with quantum dot light‐emitting diodes. This versatile, multi‐material approach enables seamless integration of device classes, paving the way for fully 3D printed next‐generation multifunctional electronic systems.

## Linked entities

- **Chemicals:** poly(vinylidene fluoride-co-trifluoroethylene) (PubChem CID 3082294), PVDF-TrFE (PubChem CID 3082294)

## Full-text entities

- **Chemicals:** PVDF-TrFE (-)
- **Species:** Homo sapiens (human, species) [taxon 9606]

## Full text

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## Figures

5 figures with captions in the complete paper: https://tomesphere.com/paper/PMC12921551/full.md

## References

62 references — full list in the complete paper: https://tomesphere.com/paper/PMC12921551/full.md

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Source: https://tomesphere.com/paper/PMC12921551