# Low-Field Optical Polarization in Type-II Quantum Dots via Nuclear-Driven Dark State Mixing

**Authors:** Gabriel M. Jacobsen, Vinicius A. de Oliveira, Baolai Liang, Morgan E. Ware, Gregory J. Salamo, Gilmar E. Marques, Yuriy I. Mazur, Victor Lopez-Richard, Marcio D. Teodoro

PMC · DOI: 10.1021/acs.nanolett.5c05163 · 2025-12-22

## TL;DR

This paper explores how weak magnetic fields can control light polarization in type-II quantum dots, offering a new approach for creating compact sources of circularly polarized light.

## Contribution

The study introduces low-field optical polarization in type-II quantum dots via nuclear-driven dark state mixing.

## Key findings

- Low magnetic fields as low as 0.17 T enable optical polarization in type-II In(Ga)As/GaAsSb QDs.
- Nuclear spin interactions mediate in-plane electron spin precession, confirmed by polarization recovery measurements.
- A theoretical model accurately reproduces the observed mirror-symmetric luminescence helicity.

## Abstract

Semiconductor quantum dots (QDs) offer a rich landscape
for spin
control and quantum light emission. While most studies have focused
on type-I band alignment, the potential of type-II systems remains
underexplored. Here, we report low-field optical polarization in type-II
In­(Ga)­As/GaAsSb QDs, enabled by hyperfine-induced mixing between bright
and dark excitons via level anticrossing under magnetic fields as
low as 0.17 T. The weak-field regime arises from the suppressed wave
function overlap, yielding a reduced electron–hole exchange
interaction. A theoretical model based on the spin Hamiltonian and
the spin-split state populations accurately captures the observed
mirror-symmetric luminescence helicity, reproducing the experimental
polarization response. Additionally, polarization recovery measurements
confirm the role of nuclear spin interactions in mediating the in-plane
electron spin precession. Our work demonstrates an alternative route
for light polarization control using weak magnetic fields and nonresonant
linear excitation, establishing type-II QDs as promising platforms
for compact sources of circularly polarized light.

## Full-text entities

- **Chemicals:** II QDs (-)

## Figures

13 figures with captions in the complete paper: https://tomesphere.com/paper/PMC12810464/full.md

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Source: https://tomesphere.com/paper/PMC12810464