# High-temperature epitaxial growth of tantalum nitride thin films on MgO: structural evolution and potential for SQUID applications

**Authors:** Michelle Cedillo Rosillo, Oscar Contreras López, Jesús Antonio Díaz, Agustín Conde Gallardo, Harvi A Castillo Cuero

PMC · DOI: 10.3762/bjnano.16.53 · Beilstein Journal of Nanotechnology · 2025-05-22

## TL;DR

This paper studies how to grow high-quality superconducting tantalum nitride films on MgO substrates using a laser technique, achieving smooth surfaces and good superconducting properties.

## Contribution

The study demonstrates the successful use of pulsed laser deposition to produce high-quality TaN superconducting films with controllable properties.

## Key findings

- TaN films deposited at 750 and 850 °C show excellent crystallinity and smooth surfaces.
- Films exhibit superconducting transition temperatures between 5.0 and 6.3 K.
- Low residual resistivity ratios confirm the high quality of the TaN films.

## Abstract

The growth of superconducting tantalum nitride (TaN) thin films on magnesium oxide (MgO) substrates has been studied using pulsed laser deposition (PLD). This research investigates the influence of varying deposition parameters, including substrate temperature and ambient gas composition, on the structural, morphological, and superconducting properties of the films. X-ray photoelectron spectroscopy, X-ray diffraction, atomic force microscopy, and transmission electron microscopy analyses revealed that the TaN films exhibit excellent crystallinity and smooth surface morphology, when deposited at optimal temperatures of 750 and 850 °C. The films exhibit superconducting transition temperatures (Tc) ranging from 5.0 to 6.3 K, depending on the stoichiometry and deposition conditions. Resistance–temperature curves further confirm the high quality of the films, as evidenced by their low residual resistivity ratios. These findings demonstrate that PLD is a suitable technique for producing high-quality TaN superconducting films.

## Linked entities

- **Chemicals:** tantalum nitride (PubChem CID 82832), magnesium oxide (PubChem CID 14792)

## Full-text entities

- **Chemicals:** MgO (MESH:D008277), TaN (-)

## Full text

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## Figures

7 figures with captions in the complete paper: https://tomesphere.com/paper/PMC12117206/full.md

## References

24 references — full list in the complete paper: https://tomesphere.com/paper/PMC12117206/full.md

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Source: https://tomesphere.com/paper/PMC12117206