Optical signatures of antiferromagnetic correlations in a strongly interacting quantum Hall MoSe2 monolayer

TL;DR

This study uses magneto-optical spectroscopy to reveal unconventional quantum Hall states in a MoSe2 monolayer, showing antiferromagnetic correlations and a zero valley polarization ground state in a strongly interacting electron liquid.

Contribution

It demonstrates the presence of antiferromagnetic interactions and unpolarized quantum Hall states in a strongly correlated MoSe2 monolayer, challenging conventional ferromagnetic models.

Findings

Observation of LL oscillations indicating correlated electron liquid behavior

Density-dependent LL crossings between valleys

Evidence of antiferromagnetic interactions favoring unpolarized states

Abstract

Strong magnetic fields quench the kinetic energy of electrons, leading to the formation of flat energy bands, known as Landau levels (LLs). In this situation, even weak interactions can drive the emergence of various ordered phases. The simplest of such phases is a quantum Hall ferromagnet, where a spontaneous spin polarization emerges when LLs with opposite spins cross. The presence of strong electron-electron interaction at zero field changes this picture and makes the resulting states much harder to predict. Here we use magneto-optical spectroscopy to reveal quantum Hall states with unconventional correlations favouring an unpolarized state in the strongly correlated electron liquid in a MoSe2 monolayer. The oscillations of the exciton polaron energies as a function of perpendicular magnetic field and electron density demonstrate the emergence of LLs in a correlated electron liquid and density-dependent crossings between LLs of opposite valleys. On lowering the LL filling factor, where interactions within LLs are stronger, the crossings systematically broaden, indicating an increase in the Zeeman energy required to fully polarize the valley-degenerate LLs. These observations are shown to be consistent with antiferromagnetic interactions between LL electrons, favouring a ground state with zero valley polarization, and are therefore inconsistent with conventional quantum Hall ferromagnetism. This discovery demonstrates a qualitatively distinct form of quantum Hall magnetism in a strongly correlated electron liquid, establishing an anchoring point for understanding spin-unpolarized fractional and ordered states of correlated electrons driven by magnetic field.