Orbital and Spin Nernst Effects in Monolayers of Transition Metal Dichalcogenides

TL;DR

This paper demonstrates that monolayer transition metal dichalcogenides can exhibit orbital and spin Nernst effects, with analytical and numerical methods revealing their dependence on doping and spin-orbit coupling.

Contribution

It introduces the orbital Nernst effect in monolayer TMDs, analyzes its mechanisms, and explores how doping and spin-orbit coupling influence these effects.

Findings

Orbital Nernst effect occurs without spin-orbit coupling.

Spin Nernst effect scales with spin-orbit strength.

Both effects are intrinsic in metallic NbS₂.

Abstract

In recent years, orbitronic effects have attracted growing attention as complementary counterparts to the well-established spintronic phenomena. In this work, we demonstrate that monolayers of transition metal dichalcogenides provide an excellent platform for the observation of the orbital Nernst effect, a relatively less explored phenomenon describing the generation of a transverse orbital current in response to an applied temperature gradient. We show that, similar to its electrical counterpart, viz., the orbital Hall effect, the orbital Nernst effect does not require the presence of spin-orbit coupling. Analytical results based on a low-energy valley model offer key insights into the underlying mechanisms, highlighting in particular the crucial role of electronic states at the Fermi energy for the emergence of this effect. The inclusion of spin-orbit coupling further gives rise to a spin Nernst effect, which scales with the strength of spin-orbit coupling and vanishes in its absence. We substantiate our analytical findings with full Brillouin-zone tight-binding results for two representative systems, monolayer 2H MoS$_2$ and 2H NbS$_2$. Our results show that while both orbital and spin Nernst conductivities in MoS$_2$ require electron or hole doping, both effects are intrinsically present in metallic NbS$_2$. Our work reveals the central role of orbital and spin Berry curvatures, identifies doping as an effective route for tuning orbital and spin Nernst responses, and proposes a possible experimental setup for detecting these effects in monolayer transition metal dichalcogenides.