Adhesion-controlled sliding and the Stribeck curve in hydrophobic soft contacts

TL;DR

This study investigates how adhesion influences sliding behavior and the Stribeck curve in hydrophobic soft contacts, revealing adhesion's role in altering contact modes beyond classical lubrication theories.

Contribution

It combines experimental and theoretical analysis to show that adhesion can induce distinct sliding modes and modify the Stribeck curve in soft hydrophobic contacts, especially on smooth surfaces.

Findings

Stribeck curves for sandblasted surfaces fit mean-field mixed-lubrication theory.

Smooth surfaces exhibit adhesion-controlled sliding with Schallamach-wave-like instabilities.

Adhesion affects contact area and sliding mode, not just fluid flow and load sharing.

Abstract

We present an experimental and theoretical study of dry and glycerol-lubricated sliding for polymethyl methacrylate (PMMA) cylinders with different surface roughness sliding on polydimethylsiloxane (PDMS) rubber. This system represents a hydrophobic soft contact, where adhesion may persist even in the presence of the lubricant and thereby modify both the real contact area and the sliding response. Dry-friction measurements, combined with contact-area calculations that include adhesion, provide a baseline for the lubricated study. For the two sandblasted surfaces, the measured Stribeck curves are described reasonably well by a mean-field mixed-lubrication theory with a fitted velocity-independent effective interfacial shear stress. In contrast, the smooth surface exhibits qualitatively different behavior. We attribute this to an adhesion-controlled sliding mode involving macroscopic Schallamach-wave-like instabilities at low sliding speeds, which are progressively suppressed as the sliding speed increases and forced wetting reduces direct solid-solid contact. The results show that, for soft hydrophobic contacts, the Stribeck curve cannot always be understood from classical fluid flow and load sharing alone. For sufficiently smooth and adhesive surfaces, adhesion changes not only the real contact area but also the sliding mode itself.