Emergent flocking dynamics in chemorepulsive active colloids: interplay of disorder and noise

TL;DR

This study explores how chemorepulsive active colloids exhibit emergent flocking behavior influenced by disorder and noise, revealing phase transitions and the importance of interaction range.

Contribution

It introduces a detailed analysis of phase transitions in chemorepulsive colloids considering quenched disorder, noise, and interaction range effects, which was not previously studied.

Findings

Phase transitions depend on noise and density, but not on pinning fraction.

Short-range interactions lead to density band formation and bimodal order parameter distribution.

Finite-size effects influence the nature of the phase transitions.

Abstract

Recent studies of active colloidal matter have revealed that a global polar order can arise from chemorepulsive interactions among particles without any explicit alignment interaction between them. In this work, we investigate such chemically interacting active colloids in the presence of quenched disorder, where a fraction of particles are randomly pinned in space. These pinned particles are restricted to rotational motion while remaining chemically coupled to the mobile population. In addition, angular noise is incorporated into the rotational dynamics to capture stochastic effects. To elucidate the interplay of quenched disorder and noise, we construct phase diagrams based on polar order and its fluctuations, and systematically analyze the associated disorder- and noise-driven phase transitions. Surprisingly, we find that the phase transition driven by the noise is significantly dependent on the density of the particles, whereas such a density-dependence is not present when the control parameter is the pinning fraction. The finite-size effects on these transitions are also examined. An effective interaction range, governed by the coefficient related to screening of the chemorepulsive interaction, plays a crucial role in collective behavior. When the effective interaction range is much smaller than the system size, the system exhibits density band formation, a feature absent in the long-range interaction regime. Moreover, near the transition point, the order parameter distribution becomes bimodal for the case of short-range interaction.