Observation and Control of Moir\'e-Tailored Topological Dirac States

TL;DR

This study provides direct spectroscopic evidence of topologically protected moiré-Dirac states in heterostructures, demonstrating control over their properties via moiré lattice tuning, advancing the understanding of topological phenomena in engineered materials.

Contribution

First direct observation of moiré-dressed Dirac states with topological character using angle-resolved photoemission spectroscopy, revealing their robustness and tunability in heterostructures.

Findings

Observation of moiré-Dirac quasiparticles with topological nodal lines.

Electrons propagate anisotropically with massless Dirac dispersion.

Topological states are protected by non-symmorphic symmetry and tunable via moiré periodicity.

Abstract

Moir\'e heterostructures provide a powerful framework for tailoring electronic band structures via controlled long-range periodic superlattice potentials. Beyond widely studied moir\'e-tailored flat bands, folded band structures can host emergent Dirac states, which have recently attracted considerable interest. Direct momentum-resolved observation of gapless moir\'e-Dirac quasiparticles, however, is challenging and has so far remained elusive. By performing angle-resolved photoemission spectroscopy measurements on an epitaxial surface-moir\'e structure, we here provide direct spectroscopic evidence of moir\'e-dressed Dirac states with topological character. Driven by the one-dimensional superlattice potential, electrons propagate anisotropically with a weak but massless Dirac dispersion along the confinement direction. The observed band crossings belong to topological nodal lines pinned to the mini-Brillouin zone boundaries. As such, they are enforced and robustly protected by the non-symmorphic symmetry of the superlattice. Finally, we demonstrate that the topological excitations can be almost continuously controlled by tuning the moir\'e lattice periodicity, directly unveiling moir\'e heterostructures as a promising platform for creating and controlling topological moir\'e-Dirac states.