Strain-Mediated Lattice Reconstruction Enhances Ferromagnetism in Cr2Ge2Te6/WTe2 van der Waals Heterobilayers

TL;DR

This study demonstrates that strain-induced lattice reconstruction at interfaces in Cr2Ge2Te6/WTe2 heterostructures significantly enhances ferromagnetism, increasing Curie temperature and coercivity through interfacial charge transfer and lattice distortions.

Contribution

It reveals that strain-mediated lattice reconstruction can be used to engineer high-temperature magnetic order in 2D vdW heterostructures, advancing magnetic device design.

Findings

Curie temperature more than doubled in heterostructures

Anomalous Hall effect observed across multiple WTe2 thicknesses

Interfacial charge transfer and lattice distortions enhance ferromagnetism

Abstract

Van der Waals (vdW) heterostructures enable tailored electronic and magnetic phases by stacking atomically thin layers with pristine interfaces. Here, we investigate fully 2D Cr2Ge2Te6/WTe2 heterostructures and identify a strong enhancement of ferromagnetism in Cr2Ge2Te6 (CGT). Magnetotransport measurements across multiple devices with WTe2 thicknesses ranging from monolayer to bulk reveal a robust anomalous Hall effect together with a more than twofold increase of the Curie temperature and substantially enhanced coercive fields. Interface microscopy confirms chemically abrupt vdW interfaces with no detectable interdiffusion, while control experiments rule out processing- or stray-field-induced artifacts. Our experiments and theoretical calculations demonstrate that interfacial charge transfer renders CGT conductive and that proximity-induced lattice distortions in CGT enhance exchange and magnetocrystalline anisotropy. These results establish strain-mediated lattice reconstruction as a strategy for engineering high-temperature magnetic order in 2D heterostructures and clarify that modifications within the magnetic layer itself can govern proximity effects in vdW stacks.