Elasticity reshapes heat flow in graphene

TL;DR

This paper demonstrates that elastic effects in graphene significantly influence heat flow by restoring phonon quasiparticles and reducing scattering, thereby enhancing thermal conductivity and phonon hydrodynamics.

Contribution

It reveals how elastic bending rigidity renormalization in graphene alters phonon scattering, linking macroscopic elasticity to microscopic thermal transport mechanisms.

Findings

Elastic bending rigidity renormalization restores phonon quasiparticles.

Reduced Umklapp scattering enhances thermal conductivity.

Strengthened phonon hydrodynamics in suspended graphene.

Abstract

Classical thermal transport theories that preserve rotational symmetry, predict strong anharmonic scattering of out-of-plane lattice vibrational modes called flexural phonons in flat suspended graphene sheets. Such strong scattering processes cause a breakdown of the phonon quasiparticle picture, which remains valid only when several cycles of lattice vibrations occur before the mode decays. Here we show that the renormalization of elastic bending rigidity ($D$), caused by the coupling between the in-plane and the out-of-plane thermal lattice fluctuations, restores phonon quasiparticles in suspended graphene. Importantly, this $D$-renormalization weakens the momentum-dissipating Umklapp phonon scattering processes, resulting in improved thermal conductivity and amplified phonon hydrodynamics in suspended graphene. Our results unveil a previously-unrecognized connection between the macroscopic elasticity and the microscopic flexural phonon scattering in two-dimensional (2D) materials that does not occur in three-dimensional bulk crystals, thereby motivating a re-examination of the classical theories and opening up new avenues to engineer the thermal as well as the phonon-limited electronic transport and relaxation in two- and lower-dimensional materials.