Mott Intermittency at the Metal-Insulator Boundary

TL;DR

This paper demonstrates that near the resistivity maximum in a Mott system, charge transport is dominated by intrinsic mesoscopic fluctuations between metallic and insulating states, indicating true phase coexistence rather than a simple crossover.

Contribution

It provides direct evidence of intrinsic metal-insulator coexistence at the resistivity maximum through time-domain transport measurements, revealing Mott intermittency as a stochastic domain switching phenomenon.

Findings

Observation of random-telegraph switching in resistance near T_max

Evidence for intrinsic phase coexistence in Mott systems

Transport governed by stochastic domain dynamics

Abstract

The resistivity maximum at a temperature $T=T_{\mathrm{max}}$ is a recurring feature of bandwidth-tuned Mott systems, yet its meaning remains controversial: is it a coherence-incoherence crossover of an electronically homogeneous metal, or does it mark the onset of transport through a mixed landscape of metallic and insulating regions? Even more debated is whether a true phase-coexistence regime survives in the relevant parameter range, or whether apparent inhomogeneity is merely extrinsic. Here we address these questions by moving beyond temperature sweeps and probe charge transport in the time domain. Near $T=T_{\mathrm{max}}$, we find that the resistance of a model system, a quasi-two-dimensional Mott spin liquid material, exhibits clear random-telegraph switching between discrete levels over long timescales. The statistics of the switching - sharp two-level behavior with thermally activated dwell times - point to a mesoscopic "current-controlling" region that dynamically toggles between metallic and insulating states, intermittently opening and closing the dominant conduction channel. This characteristic fluctuating dynamics provides direct evidence for intrinsic metal-insulator coexistence and establishes $T\sim T_{\mathrm{max}}$ as the regime of Mott intermittency, where transport is governed by stochastic domain switching rather than quasiparticle decoherence.