Limitations of an approximative phase-space description in strong-field quantum optics

TL;DR

This paper critically examines the limitations of an approximate phase-space method in modeling quantum optical properties in strong-field processes like high-order harmonic generation, revealing it can mischaracterize quantum features such as squeezing and photon statistics.

Contribution

It introduces and evaluates the accuracy of an approximate phase-space description in strong-field quantum optics, highlighting its shortcomings in capturing quantum optical observables.

Findings

The approximation mischaracterizes the quantum optical properties of the driving laser.

It fails to predict sub-Poissonian photon statistics and quadrature squeezing.

The error scales with pulse duration and emitter density.

Abstract

In recent years, strong-field processes such as high-order harmonic generation (HHG) and above-threshold ionization driven by nonclassical states of light have become an increasingly popular field of study. The theoretical modeling of these processes often applies an approximate phase-space expansion of the nonclassical driving field in terms of coherent states, which has been shown to accurately predict the harmonic spectrum. However, its accuracy for the computation of quantum optical observables like the degree of squeezing and photon statistics has not been thoroughly considered. In this work, we introduce this approximative phase-space description and discuss its accuracy, and we find that it mischaracterizes the quantum optical properties of the driving laser by making it an incoherent mixture of classical states. We further show that this error in the driving field description maps onto the light emitted from HHG, as neither sub-Poissonian photon statistics nor quadrature squeezing below vacuum fluctuations can be captured by the approximative phase-space description. Lastly, to benchmark the approximative phase-space description, we consider the quantum HHG from a one-band model, which yields an exact analytical solution. Using the approximative phase-space representation with this specific model, we find a small quantitative error in the quadrature variance of the emitted field that scales with pulse duration and emitter density. Our results show that using this approximative phase-space description can mischaracterize quantum optical observables. Attributing physical meaning to such results should therefore be accompanied by a quantitative analysis of the error.