Electronic Origin of Density Wave Orders in a Trilayer Nickelate

TL;DR

This study investigates the electronic structure of trilayer Ruddlesden-Popper nickelate La$_4$Ni$_3$O$_{10}$, revealing the origin of magnetic order and its implications for high-temperature superconductivity.

Contribution

First experimental evidence of band splitting due to interlayer coupling and identification of Fermi surface nesting as the origin of magnetic order in La$_4$Ni$_3$O$_{10}.

Findings

Band splitting induced by interlayer coupling

Momentum-dependent density wave gap structures

Mirror-selective Fermi surface nesting causes antiferromagnetic order

Abstract

The discovery of superconductivity in Ruddlesden-Popper nickelates has established a new frontier in the study of high-temperature superconductors. However, the underlying pairing mechanism and its relationship to the material's electronic and magnetic ground states remain elusive. Since unconventional superconductivity often emerges from a complex interplay of magnetic correlations, elucidating the magnetic ground state of the nickelates at ambient pressure is crucial for understanding the emergence of superconductivity under high pressure. Here, we combine high-resolution angle-resolved photoemission spectroscopy with tight-binding model simulation to investigate the electronic structure of the representative trilayer Ruddlesden-Popper nickelate La$_4$Ni$_3$O$_{10}$. We provide the first experimental evidence of band splitting induced by interlayer coupling and further resolve the momentum-dependent density wave gap structures along all the Fermi surfaces. Our findings identify the mirror-selective Fermi surface nesting as the origin of the interlayer antiferromagnetic spin density wave and demonstrate the dominant role of Ni-3d$_{z^2}$ orbitals in the low-energy physics of La$_4$Ni$_3$O$_{10}$. These results provide a fundamental framework for understanding the magnetic interactions and high-temperature superconductivity mechanism in the Ruddlesden-Popper nickelate family.