Spectral properties of high-order harmonic radiation enhanced by XUV-driven electron-hole dynamics

TL;DR

This paper investigates how high-order harmonic spectra extend beyond the usual cutoff by analyzing the effects of XUV-driven electron-hole dynamics and their sensitivity to experimental parameters.

Contribution

It introduces a detailed analysis of the spectral properties of extended high-order harmonics influenced by XUV and IR pulse interactions, highlighting phase sensitivity and coherence effects.

Findings

Spectral extension depends on IR-XUV delay and IR intensity.

Signal strength diminishes with chirped XUV pulses and poor coherence.

Decoherence among emitters can suppress harmonic signals.

Abstract

We analyze the spectral properties of high-order harmonic radiation with photon energies extending beyond the regular cutoff energy in standard high-order harmonic generation. The extension of the regular harmonic cutoff results from infrared (IR)-driven recombination of valence photoelectrons into a cationic core hole created by extreme-ultraviolet (XUV) excitation of inner-shell electrons into the transient valence hole in a combined XUV+IR configuration [Buth et al., Opt. Lett. 36, 3530 (2011)]. We show that the microscopic dipole phase at the extended harmonic frequencies is sensitive to the relative IR-XUV delay and IR intensity, whereas the corresponding signal intensity drops significantly for chirped XUV pulses with poor temporal coherence. We discuss the impact of such sensitivity on the macroscopic harmonic radiation, whereby decoherence among the dipole emitters may lead to further signal suppression.