Quantum control of Hubbard excitons

TL;DR

This paper demonstrates the use of Floquet engineering to achieve quantum control of a strongly correlated Hubbard exciton in a 1D Mott insulator, enabling ultrafast state manipulation with potential for quantum sensing.

Contribution

It introduces a method to coherently dress and rotate many-body exciton wavefunctions in a solid-state system using nonresonant optical fields, advancing quantum control techniques.

Findings

Achieved ultrafast $a/2$ rotations of exciton states

Quantified control using resonant third-harmonic generation

Demonstrated manipulation of strongly correlated excitons

Abstract

Quantum control of the many-body wavefunction is a central challenge in quantum materials research, as it could yield a precise control knob to manipulate emergent phenomena. Floquet engineering, the coherent dressing of quantum states with periodic non-resonant optical fields, has become an important strategy for quantum control. Most applications to solid-state systems have targeted weakly interacting or single-ion states, leaving the manipulation of many-body wavefunctions largely unexplored. Here, we use Floquet engineering to achieve quantum control of a strongly correlated Hubbard exciton in the one-dimensional Mott insulator Sr$_2$CuO$_3$. A nonresonant midinfrared optical field coherently dresses the exciton wavefunction, driving its rotation between bright and dark states. We use resonant third-harmonic generation to quantify ultrafast $\pi/2$ rotations on the Bloch sphere spanned by these exciton states. Our work advances the quest towards programmable control of correlated states and exciton-based quantum sensing.