Coupling Quantum Dots to Elastic Waves in a Phononic Crystal Waveguide

TL;DR

This paper investigates how quantum dots couple to elastic waves in phononic crystal waveguides, revealing mode-dependent mechanisms and potential for quantum device applications through detailed simulations.

Contribution

It combines multiband kp and configuration-interaction simulations with finite-element modeling to analyze QD-phonon interactions, identifying dominant coupling channels and their signatures.

Findings

Energy shifts up to 0.7 meV under acoustic waves

Quadratic responses cause frequency doubling

Mode symmetries dictate coupling mechanisms

Abstract

We present a comprehensive study of quantum dot (QD) coupling to various phononic modes in a phononic waveguide, combining multiband kp and configuration-interaction (CI) QD state simulations with finite-element waveguide mode modeling. We consider self-assembled Stranski-Krastanov InGaAs/GaAs as well as local droplet-etched GaAs/AlGaAs structures. Using kp-CI calculations, we quantify the strain and piezoelectric responses of InAs and GaAs QDs. By systematically isolating volumetric/shear deformation-potential and piezoelectric channels, we demonstrate how mode symmetries dictate distinct coupling mechanisms. We identify the dominant coupling channels and characterize their observable signatures in the QD response. We predict strong linear energy shifts under volumetric strain and quadratic behavior under shear strain, especially in GaAs QDs. The piezoelectric effect is dominated by polarizability, which also leads to a quadratic response. The simulations show energy modulations up to 0.7 meV for an acoustic wave with 0.1 nm amplitude. The quadratic response to shear strain and piezoelectric field leads to frequency doubling in the QD response to a mechanical wave and to non-harmonic time traces when linear and quadratic effects contribute to a similar degree. The deep understanding of QD-acoustic couplings opens pathways to the optimal design of QD and waveguide structures, as well as to improved engineering of acousto-optic quantum interfaces.