Quenching the Non-Collinear Spin Order in High-Tc Layered Ferromagnet Fe5GeTe2

TL;DR

This study investigates the magnetic phase transition in Fe5GeTe2, revealing a switch from collinear to non-collinear order near 160K, and demonstrates that Ni substitution can quench this non-collinear spin order, advancing 2D magnetic device development.

Contribution

It uncovers the mechanism behind non-collinear spin order in Fe5GeTe2 and shows Ni substitution as an effective method to quench this order, offering new control over 2D magnetism.

Findings

Magnetic transition from collinear to non-collinear near 160K.

Ni substitution suppresses non-collinear spin order.

Insights into magnetism of high-Tc layered ferromagnets.

Abstract

The realization of long-range spin order in two-dimensions (2D) has catapulted the search for layered materials with magnetic ordering above room temperature. These efforts aim to understand and enhance the spin spin interactions in 2D. An emergent class of such magnets is the layered FeNGeTe2 (N = 3, 4, and 5). Here, we investigate the magnetic states over a wide field temperature phase space in the high-Tc ferromagnet Fe5GeTe2 using magnetization, ferromagnetic resonance (FMR), and magneto-transport measurements. Our findings reveal a magnetic phase transition from a collinear to a complex non-collinear magnetic order near the temperature T* = 160 K, below which magnetic susceptibility is reduced, FMR linewidth broadened, and anomalous Hall resistivity suppressed. Such non-collinearity results from the competition between magnetocrystalline anisotropy and Dzyaloshinskii Moriya interaction arising from the unusual Fe1 ordering in two possible split sites. Our study focuses on the strategy to quench the non-collinear spin order. Substituting 40% Ni in Fe5GeTe2 is found to be one such quenching strategy. This provides deeper insights into the magnetism of a high-Tc layered-ferromagnet, offering opportunities to develop 2D magnet-based devices.