Laser-Induced Current Transients in Ultrafast All-Optical Switching of Metallic Spin Valves

TL;DR

This paper models laser-induced current transients in ultrafast all-optical switching of metallic spin valves, highlighting the role of spin-polarized hot electron currents and their dynamics in switching behavior.

Contribution

It introduces a comprehensive atomistic spin drift-diffusion model that captures the effects of superdiffusive and diffusive electron flows during optical switching.

Findings

Switching is driven mainly by spin-polarized hot electron currents.

Initial superdiffusive forward flow causes parallel to antiparallel switching.

Backward diffusive flow influences multi-domain formation at higher fluences.

Abstract

All-optical switching in a ferromagnetic spin valve is studied here using atomistic spin drift-diffusion dynamics, which includes contributions from spin pumping and superdiffusive transport. We find the switching is governed principally by spin-polarized currents due to non-equilibrium hot electrons excited by the laser pulse and re-equilibration currents. In particular, an initial superdiffusive forward flow of electrons, polarized by the free layer, is generated. This drives parallel to antiparallel switching of the free layer through accumulation of minority spins at the reference layer. A diffusive backward flow of electrons, repolarized by the reference layer, follows the initial superdiffusive flow as the charge distribution re-equilibrates. Due to the pulse width-dependent asymmetric amplitudes of the forward and backward transients, the latter can drive antiparallel to parallel switching, and create multi-domain structures at higher laser fluences and longer pulses. The results obtained here are in agreement with experimental observations, providing a framework for self-consistent modelling of all-optical switching in metallic heterostructures.