Anomalous Hall effect and rich magnetic phase diagram of Mn$_{100-x}$Rh$_{x}$ epitaxial films

TL;DR

This study explores the magnetic phases and anomalous Hall effect in Mn$_{100-x}$Rh$_x$ epitaxial films, revealing a complex phase diagram and strong links between magnetic order and electronic topology, with potential for antiferromagnetic spintronics.

Contribution

It provides the first systematic investigation of magnetic phase transitions and Hall effects in Mn-Rh thin films with optimized epitaxial growth, uncovering rich magnetic behavior and electronic correlations.

Findings

Identification of three magnetic regimes depending on Rh content.

Observation of a strong anomalous Hall effect linked to Berry curvature.

Correlation between electronic transport properties and magnetic phases.

Abstract

A series of Mn$_{100-x}$Rh$_x$ ($20 \le x \le 50$) thin films were epitaxially grown on the MgO substrate using magnetron sputtering technique, and were systematically investigated by magnetization, longitudinal electrical resistivity, and transverse Hall resistivity. After optimizing the growth conditions, phase-pure Mn$_{100-x}$Rh$_x$ films with a cubic CsCl-type structure were obtained, and their magnetic phase diagram was built. The manipulation of Rh content leads to a rich magnetic phase diagram, where three different regimes can be identified: for $x < 40$, Mn$_{100-x}$Rh$_x$ films undergo a ferromagnetic (FM) transition below $T_\mathrm{C} \approx$ 330-350 K; for $40 \le x \le 45$, in addition to the FM transition at $T_\mathrm{C} \approx$ 200 K, Mn$_{100-x}$Rh$_x$ films undergo a FM-to-antiferromagnetic (AFM) transition at $T_\mathrm{N} \approx$ 120 K; finally for $x > 45$, only one AFM transition at $T_\mathrm{N} \approx$ 150 K can be tracked. All the Mn$_{100-x}$Rh$_x$ films exhibit distinct anomalous Hall effect in their magnetically ordered state, which is most likely due to the intrinsic Berry-curvature mechanism. In addition, all the anomalous Hall transport properties, including the resistivity, conductivity, and angle exhibit a strong correlation with the magnetic properties of Mn$_{100-x}$Rh$_x$ films, which become most evident for $x$ = 35. Our systematic investigations suggest a strong correlation between magnetic properties and electronic band topology in Mn$_{100-x}$Rh$_x$ films, highlighting their great potential for AFM spintronics.