Low-dimensionality-induced tunable ferromagnetism in SrRuO$_3$ ultrathin films

TL;DR

This study demonstrates how low-dimensional quantum states in ultrathin SrRuO$_3$ films enable precise tuning of ferromagnetism by controlling the density of states, with implications for designing customizable quantum materials.

Contribution

It reveals that ferromagnetism in SrRuO$_3$ ultrathin films can be tuned through DOS control at a phase crossover, combining experimental and theoretical insights.

Findings

Spin-split band structure visualized via SRPES/ARPES

Magnetism modulated by electron doping across high-DOS point

Establishment of a pathway for designing tunable quantum materials

Abstract

Quantum materials near electronic or magnetic phase boundaries exhibit enhanced tunability, as their emergent properties become highly sensitive to external perturbations. Here, we demonstrate precise control of ferromagnetism in a SrRuO$_3$ ultrathin film, where a high density of states (DOS), arising from low-dimensional quantum states, places the system at the crossover between a non-magnetic and bulk ferromagnetic state. Using spin- and angle-resolved photoemission spectroscopy (SRPES/ARPES), transport measurements, and theoretical calculations, we systematically tune the Fermi level via electron doping across the high-DOS point. We directly visualize the spin-split band structure and reveal its influence on both magnetic and transport properties. Our findings provide compelling evidence that magnetism can be engineered through DOS control at a phase crossover, establishing a pathway for the rational design of tunable quantum materials.