Saturation Field as a Direct Probe of Exchange and Single-Ion Anisotropies in Spin-1 Magnets

TL;DR

This paper demonstrates that the saturation field in spin-1 magnets can directly reveal exchange and single-ion anisotropies, offering a practical method for probing microscopic magnetic properties through high-field experiments.

Contribution

We derive analytic expressions for magnon spectra and critical fields in spin-1 systems using the SU(3) bond operator framework, linking saturation fields to anisotropy parameters.

Findings

Upper critical field $h_{c2}$ indicates exchange and single-ion anisotropies.

Magnon Bose Einstein condensation dome is influenced by anisotropies and interlayer coupling.

Criteria for identifying symmetry breaking mechanisms in spin-1 materials are provided.

Abstract

High magnetic fields provide a direct route to probe the anisotropies that govern spin dynamics in layered magnets. Using the SU(3) bond operator framework for spin 1 systems, we derive analytic expressions for the magnon spectrum and the critical fields delimiting the field induced ordered phase. We show that the upper critical field $h_{c2}$ carries a simple and quantitative fingerprint of both exchange anisotropy and single ion symmetry breaking, enabling high field experiments to serve as sensitive probes of microscopic anisotropy. We further map how these anisotropies, together with interlayer coupling, control the extent and location of the magnon Bose Einstein condensation dome. Our results provide experimentally accessible criteria for identifying symmetry breaking mechanisms in real spin 1 materials.