New insights into the magnetism of DyCo$_{5}$

TL;DR

This study provides the first detailed magnetization measurements of DyCo$_{5}$ single crystals up to 600 K and 14 T, revealing complex magnetic behavior and anisotropy, explained through advanced theoretical modeling.

Contribution

It introduces comprehensive experimental data on DyCo$_{5}$ magnetism and develops a theoretical framework that explains its temperature-dependent magnetic properties.

Findings

Identification of significant magnetization anisotropy.

Observation of a minimum in spontaneous magnetization near the compensation point.

Successful theoretical reproduction of experimental magnetic behavior.

Abstract

In this work, we present the first magnetization measurements of DyCo$_5$ single crystals in magnetic fields up to 14 T, spanning a temperature range up to 600 K. Our investigation reveals several unique features, including a significant magnetization anisotropy and an observed minimum in spontaneous magnetization near the compensation point, phenomena not previously reported. This work also uncovers the complex magnetic behavior of DyCo$_5$, with a pronounced interplay between the Dy and Co sublattices, each exhibiting distinct temperature-dependent magnetic properties. The combination of dynamical mean-field theory (DMFT), atomistic spin-dynamics (ASD) simulations, and the Effective Spin Model (ESM) for rare-earth compounds successfully explains the experimental data across both low and high temperatures. Our theoretical approach not only explains the observed magnetic anisotropy and the behavior near the compensation temperature but also successfully reproduces key experimental features such as the saturation behavior at high fields and the evolution of the magnetic moment at different temperatures.