Energy-Dependent Magnetic Modifications in HOPG via Microbeam Scanning

TL;DR

This study investigates how varying ion energies influence magnetic modifications in HOPG, revealing that carbon ions at specific energies induce stronger magnetic ordering due to defect creation.

Contribution

It demonstrates the energy-dependent magnetic effects in HOPG caused by ion irradiation, highlighting the role of ion species and energy in magnetic property modification.

Findings

Carbon ion irradiation yields higher magnetic ordering than protons at the same dose.

Maximum magnetization occurs at 1.2 MeV carbon ion energy.

SRIM simulations show more lattice defects from carbon ions, correlating with increased magnetism.

Abstract

Medium-energy ion irradiation is a promising technique for inducing magnetism in materials with partially filled d or f electron bands. This approach enables precise control over the density and spatial distribution of irradiation-induced defects, which play a crucial role in modifying the electronic and magnetic properties of the system. The primary objective of this experiment was to investigate the influence of ion energy variation on the magnetic properties of highly oriented pyrolytic graphite (HOPG). To achieve this, HOPG samples were irradiated with protons 1-3 MeV and carbon ions 600 keV - 2 MeV. A significant change in the magnetic moment was observed with respect to the irradiation energy for both ion species. The effect of energy variation was analyzed using a vibrating sample magnetometer (VSM) and SRIM simulations. The results demonstrate that ion-beam-induced magnetic ordering strongly depends on both the ion species and the beam energy. Magnetic measurements were performed with varying irradiation energies, showing that carbon ion irradiation produces a higher degree of magnetic ordering compared to proton irradiation at the same dose. The maximum magnetization was obtained at 1.2 MeV carbon ion irradiation. SRIM simulations confirm that carbon ions create a greater number of lattice defects than proton ions, which correlates with the enhanced magnetic response.