Spinon excitations and spin correlations in the one-dimensional quantum magnet $\beta$-VOSO$_4$ probed by Raman spectroscopy

TL;DR

This study uses Raman spectroscopy to detect spinon excitations and analyze spin correlations in the one-dimensional quantum magnet $eta$-VOSO$_4$, demonstrating the growth of quantum correlations at low temperatures.

Contribution

It provides experimental evidence of spinon excitations in $eta$-VOSO$_4$ and introduces quantum Fisher information as a new probe for spin correlations in quantum magnets.

Findings

Detection of gapless spinon continuum along the chain direction

Temperature-dependent increase in quantum Fisher information

Agreement between experimental data and density matrix renormalization group calculations

Abstract

Fractionalized excitations such as spinons and anyons have emerged as a central theme in condensed matter physics with broad implications for superconductivity, quantum statistics, and quantum computation. The nearly ideal one-dimensional $S=1/2$ system $\beta$-VOSO$_4$ without long-range order down to 85 mK provides a promising platform to experimentally explore such fractionalized excitations. Here, we employ Raman spectroscopy to probe magnetic excitations and the evolution of spin correlations in $\beta$-VOSO$_4$. Spinon signatures are found along the chain direction, evidenced by a broad, gapless scattering continuum at low temperatures. The temperature dependence of the spinon spectral weight aligns considerably with numerical density matrix renormalization group calculations. By comparing the experimental spinon spectral weight with calculated results and evaluating the associated quantum Fisher information (QFI) therefrom, we observe a steep increase in QFI upon cooling, indicating rapidly growing correlation lengths. Our study showcases QFI as a probe of spin correlations in quantum magnets.