Bidimensional measurements of photon statistics within a multimodal temporal framework

TL;DR

This paper introduces a method for ultrafast, spatially resolved photon statistics measurement using difference-frequency generation, enabling discrimination of photon types with high temporal resolution and analyzing limitations due to multimodal effects.

Contribution

The work presents a novel single-shot, two-dimensional photon statistics measurement technique with picosecond resolution and a theoretical framework to understand measurement limitations.

Findings

Discriminates between coherent and thermal photon statistics spatially

Develops a temporal mode decomposition model matching experimental data

Identifies vacuum contamination and multimodal response as measurement limitations

Abstract

Ultrafast imaging of photon statistics in two dimensions is a powerful tool for probing non-equilibrium and transient optical phenomena, yet it remains experimentally challenging due to the simultaneous need for high temporal resolution and statistical fidelity. In this work, we demonstrate spatially resolved single-shot measurements of photon number distributions using difference-frequency generation (DFG) in a nonlinear BBO crystal. We show that our platform can discriminate between coherent and thermal photon statistics across two spatial dimensions with picosecond resolution. At the same time, we find that the retrieved distributions deviate from the ideal ones, a consequence of vacuum contamination and the multimodal response of the amplifier. To explain this, we develop a temporal mode decomposition framework that captures the essential physics of signal amplification and fluorescence, and quantitatively reproduces the experimental findings. This establishes a robust approach for measuring two-dimensional photon statistics while clarifying the fundamental factors that limit the fidelity of such measurements.